Rapid and low-cost detection of saffron ( Crocus sativus L.) adulteration using smartphone videos and spectral data fusion strategy

Saffron (Crocus sativus L.) is the most expensive spice in the world and is highly susceptible to economically motivated adulteration. Hyperspectral imaging (HSI) and near-infrared (NIR) spectroscopy are recently popular techniques for rapid, non-destructive detection of saffron adulteration. However, the high cost and measurement complexity of these techniques make them less suitable for consumer-level applications. In this work, a smartphone video-based system combined with chemometrics is used to detect saffron adulteration. A smartphone is utilised to capture short videos of pure and adulterated saffron powder samples illuminated by its colourchanging screen. The video frames are decomposed into RGB colour images and converted into spectral-like data. Partial least squares regression is used to model the relationship between data and saffron purity. The smartphone video-based system obtains a coefficient of determination of 0.9774 for prediction, which is comparable to reference techniques such as NIR spectroscopy and HSI. Moreover, it is efficient in presenting distribution maps related to saffron purity. In addition, when used in conjunction with the smartphone video-based system, HSI and NIR spectroscopy achieve higher performance without significantly increasing measurement cost and complexity. Such results suggest that the smartphone video-based system has the potential to be a viable primary screening and auxiliary tool for detecting saffron adulteration.