Enhancing Rural Surface Water Remediation with Iron-Carbon Microelectrolysis-Strengthened Ecological Floating Beds

被引:0
作者
Wang, Han [1 ]
Wang, Tianbei [1 ]
Wang, Weigang [2 ]
Yuan, Yue [3 ]
机构
[1] Tongji Univ, Coll Environm Sci & Engn, Shanghai 200092, Peoples R China
[2] Nankai Univ, Coll Environm Sci & Engn, Tianjin 300071, Peoples R China
[3] Chinese Res Inst Environm Sci, State Key Lab Environm Criteria & Risk Assessment, Beijing 100012, Peoples R China
基金
中国国家自然科学基金;
关键词
wastewater treatment; sustainable remediation; ecological floating bed; surface water; iron-carbon microelectrolysis; ADSORPTION; REDUCTION; NITRATE;
D O I
10.3390/su16177417
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Ecological floating beds, with their compact footprint and mobility, offer a promising solution for sustainable surface water remediation in rural areas. However, low removal efficiency and instability still limit its application. In this study, iron-carbon-based fillers were integrated into ecological floating beds to investigate their impact and mechanisms in removing pollutants, including carbon, nitrogen, phosphorus, and heavy metals. Results indicate that all five fillers (activated carbon, iron-carbon fillers, sponge iron, activated carbon + iron-carbon fillers, and activated carbon + sponge iron) can completely remove orthophosphate, and the sponge iron filler system can completely remove nitrate. Then, fillers were applied to ecological floating beds, and the iron-carbon microelectrolysis (activated carbon + sponge iron filler)-enhanced ecological floating bed showed superior removal efficiency for pollutants. It achieved 95% removal of NH4+-N, 85% removal of NO3--N, 75% removal of total phosphorus, 90% removal of chemical oxygen demand, and 90% removal of heavy metals. Typical nitrifying bacteria Nitrospira, denitrifying bacteria Denitratisoma, and a variety of bacterial genera with denitrification functions (e.g., Rhodobacter, Dechloromonas, Sediminibacterium, and Novosphingobium) coexisted in the system, ensuring efficient and robust nitrogen removal performance. These findings will provide support for the sustainable treatment of surface water in rural areas.
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页数:12
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共 35 条
  • [1] Enhanced reduction of nitrate by zero-valent iron at elevated temperatures
    Ahn, Se Chang
    Oh, Seok-Young
    Cha, Daniel K.
    [J]. JOURNAL OF HAZARDOUS MATERIALS, 2008, 156 (1-3) : 17 - 22
  • [2] Combination of granular activated carbon adsorption and deep-bed filtration as a single advanced wastewater treatment step for organic micropollutant and phosphorus removal
    Altmann, Johannes
    Rehfeld, Daniel
    Traeder, Kai
    Sperlich, Alexander
    Jekel, Martin
    [J]. WATER RESEARCH, 2016, 92 : 131 - 139
  • [3] Predicting Phosphorus Release from Anaerobic, Alkaline, Flooded Soils
    Amarawansha, Geethani
    Kumaragamage, Darshani
    Flaten, Don
    Zvomuya, Francis
    Tenuta, Mario
    [J]. JOURNAL OF ENVIRONMENTAL QUALITY, 2016, 45 (04) : 1452 - 1459
  • [4] Remediation of Polluted River Water by Biological, Chemical, Ecological and Engineering Processes
    Anawar, Hossain Md
    Chowdhury, Rezaul
    [J]. SUSTAINABILITY, 2020, 12 (17)
  • [5] [Anonymous], 2002, 38382002 GB
  • [6] Bojanic HA, 2017, EUROCHOICES, V16, P05, DOI 10.1111/1746-692X.12143
  • [7] Phosphorus adsorption in Fe-loaded activated carbon: Two-site monolayer equilibrium model and phenomenological kinetic description
    Braun, Julia C. A.
    Borba, Carlos E.
    Godinho, Marcelo
    Perondi, Daniele
    Schontag, Juliana M.
    Wenzel, Bruno M.
    [J]. CHEMICAL ENGINEERING JOURNAL, 2019, 361 : 751 - 763
  • [8] Iron Carbide@Carbon Nanocomposites: A Tool Box of Functional Materials
    Defilippi, Chiara
    Mukadam, Mariam Omar Ali
    Nicolae, Sabina Alexandra
    Lees, Martin Richard
    Giordano, Cristina
    [J]. MATERIALS, 2019, 12 (02)
  • [9] Heterogeneous electro-Fenton system using Fe-MOF as catalyst and electrocatalyst for degradation of pharmaceuticals
    Fdez-Sanromán A.
    Pazos M.
    Sanromán M.A.
    Rosales E.
    [J]. Chemosphere, 2023, 340
  • [10] Role of phosphate fertilizers in heavy metal uptake and detoxification of toxic metals
    Gupta, D. K.
    Chatterjee, S.
    Datta, S.
    Veer, V.
    Walther, C.
    [J]. CHEMOSPHERE, 2014, 108 : 134 - 144