Improving the ferroelectric properties of Lu doped Hf0.5Zr0.5O2 thin films by capping a CeO x layer

被引:1
作者
Xiao, Yongguang [1 ]
Yang, Lisha [1 ]
Jiang, Yong [1 ]
Liu, Siwei [1 ]
Li, Gang [1 ]
Ouyang, Jun [1 ,2 ]
Tang, Minghua [1 ]
机构
[1] Xiangtan Univ, Sch Mat Sci & Engn, Xiangtan 411105, Peoples R China
[2] Qilu Univ Technol, Shandong Acad Sci, Jinan 250353, Shandong, Peoples R China
基金
中国国家自然科学基金;
关键词
CSD; ferroelectricity; HZO; wake-up free; TRANSITION; STORAGE; ZRO2;
D O I
10.1088/1361-6528/ad5bee
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
Lu doped Hf0.5Zr0.5O2 (HZO) ferroelectric films were prepared on Pt/TiN/SiO2/Si substrate by chemical solution deposition method, and an interfacial engineering strategy for improving the ferroelectric property was explored by capping the Lu doped HZO films with a cerium oxide layer. Compared with the Lu doped HZO film without the CeOx coating layer, the Lu doped HZO film with the CeOx coating layer has a larger remanent polarization (2P(r) = 34.72 mu C cm(-2)) and presents weaker wake-up behavior, which result from the higher orthogonal phase ratio and the lower oxygen vacancy of the CeOx coated Lu doped HZO film. In addition, the CeOx coating can remarkably improve the fatigue resistance and retention performance of the Lu doped HZO films. It is hoped that the results can provide an effective approach for the realization of high-performance and highly reliable hafnium oxide based ferroelectric thin films.
引用
收藏
页数:7
相关论文
共 44 条
[1]   Ferroelectricity in hafnium oxide thin films [J].
Boescke, T. S. ;
Mueller, J. ;
Braeuhaus, D. ;
Schroeder, U. ;
Boettger, U. .
APPLIED PHYSICS LETTERS, 2011, 99 (10)
[2]  
Cai Y L., 2022, IEEE INT C EL PACK T, P1
[3]   Wake-up-free ferroelectric Hf0.5Zr0.5O2 thin films characterized by precession electron diffraction [J].
Chang, Teng-Jan ;
Chen, Hsing-Yang ;
Wang, Chin-, I ;
Lin, Hsin-Chih ;
Hsu, Chen-Feng ;
Wang, Jer-Fu ;
Nien, Chih-Hung ;
Chang, Chih-Sheng ;
Radu, Iuliana P. ;
Chen, Miin-Jang .
ACTA MATERIALIA, 2023, 246
[4]   Ferroelectric Polarization Enhancement in Hafnium-Based Oxides Through Capping Layer Engineering [J].
Chen, Hsuan-Han ;
Liao, Ruo-Yin ;
Chou, Wu-Ching ;
Hsu, Hsiao-Hsuan ;
Cheng, Chun-Hu ;
Huang, Ching-Chien .
IEEE JOURNAL OF THE ELECTRON DEVICES SOCIETY, 2022, 10 :947-952
[5]   Wake-Up Free Ferroelectric Capacitor With Quadruple-Level Storage by Inserting ZrO2 Interlayer and Bottom Layer in HfZrOx [J].
Chen, Yi-Fan ;
Hu, Chia-Wei ;
Kao, Yu-Cheng ;
Kuo, Chun-Yi ;
Wu, Pin-Jiun ;
Wu, Yung-Hsien .
IEEE ELECTRON DEVICE LETTERS, 2023, 44 (03) :400-403
[6]   Reversible transition between the polar and antipolar phases and its implications for wake-up and fatigue in HfO2-based ferroelectric thin film [J].
Cheng, Yan ;
Gao, Zhaomeng ;
Ye, Kun Hee ;
Park, Hyeon Woo ;
Zheng, Yonghui ;
Zheng, Yunzhe ;
Gao, Jianfeng ;
Park, Min Hyuk ;
Choi, Jung-Hae ;
Xue, Kan-Hao ;
Hwang, Cheol Seong ;
Lyu, Hangbing .
NATURE COMMUNICATIONS, 2022, 13 (01)
[7]   Improved Ferroelectric Switching Endurance of La -Doped Hf0.5Zr0.5O2 Thin Films [J].
Chernikova, Anna G. ;
Kozodaev, Maxim G. ;
Negrov, Dmitry V. ;
Korostylev, Evgeny V. ;
Park, Min Hyuk ;
Schroeder, Uwe ;
Hwang, Cheol Seong ;
Markeev, Andrey M. .
ACS APPLIED MATERIALS & INTERFACES, 2018, 10 (03) :2701-2708
[8]   Nanoscale Doping and Its Impact on the Ferroelectric and Piezoelectric Properties of Hf0.5Zr0.5O2 [J].
Chouprik, Anastasia ;
Kirtaev, Roman ;
Korostylev, Evgeny ;
Mikheev, Vitalii ;
Spiridonov, Maxim ;
Negrov, Dmitrii .
NANOMATERIALS, 2022, 12 (09)
[9]   Ferroelectricity and ferroelectric resistive switching in sputtered Hf0.5Zr0.5O2 thin films [J].
Fan, Zhen ;
Xiao, Juanxiu ;
Wang, Jingxian ;
Zhang, Lei ;
Deng, Jinyu ;
Liu, Ziyan ;
Dong, Zhili ;
Wang, John ;
Chen, Jingsheng .
APPLIED PHYSICS LETTERS, 2016, 108 (23)
[10]   Possible electrochemical origin of ferroelectricity in HfO2 thin films [J].
Glinchuk, Maya D. ;
Morozovska, Anna N. ;
Lukowiak, Anna ;
Strek, Wieslaw ;
Silibin, Maxim V. ;
Karpinsky, Dmitry V. ;
Kim, Yunseok ;
Kalinin, Sergei V. .
JOURNAL OF ALLOYS AND COMPOUNDS, 2020, 830