Nitrogen-doped carbon materials as a promising platform toward the efficient catalysis for hydrogen generation

被引：69

作者：

Salinas-Torres, David ^{[1
]}

Navlani-Garcia, Miriam ^{[1
]}

Mori, Kohsuke ^{[1
,2
,3
]}

Kuwahara, Yasutaka ^{[1
,2
]}

Yamashita, Hiromi ^{[1
,2
]}

机构：

[1] Osaka Univ, Grad Sch Engn, Div Mat & Mfg Sci, 2-1 Yamada Oka, Suita, Osaka 5650871, Japan

[2] Kyoto Univ, Unit Elements Strategy Initiat Catalysts & Batter, Kyoto 6152520, Japan

[3] JST, PRESTO, 4-1-8 Honcho, Kawaguchi, Saitama 3320012, Japan

来源：

APPLIED CATALYSIS A-GENERAL | 2019年 / 571卷

基金：

日本学术振兴会;

关键词：

N-doped carbon; Hydrogen production; Formic acid; Ammonia borane; Water splitting; OXYGEN REDUCTION REACTION; MACRORETICULAR ACIDIC RESIN; ORDERED MESOPOROUS CARBONS; DOUBLE-LAYER CAPACITORS; FORMIC-ACID; HIGHLY EFFICIENT; GRAPHENE OXIDE; COBALT NANOPARTICLES; SODIUM-BOROHYDRIDE; NANOPOROUS CARBONS;

D O I：

10.1016/j.apcata.2018.11.034

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Nitrogen-doped carbon materials have emerged as versatile candidates with outstanding features as both support of metal-based catalysts and metal-free catalytic systems. Their use has been traditionally linked to electro-chemical applications, but the number of applications in which these materials show their virtues has been exponentially increasing in the last decade. Particularly, catalysts based on metal nanoparticles supported on nitrogen-doped carbon materials have shown to be attractive for important catalytic reactions as they display enhanced performances endowed by well-dispersed, stabilized and electronically promoted nanoparticles as well as by the modified acid-base properties of the support. The present review is focused on the most recent breakthroughs achieved by these catalytic systems in the hydrogen production from some of the most representative hydrogen carrier molecules by highlighting the effect of the incorporation of nitrogen in the support matrix.

引用

页码：25 / 41

页数：17

共 214 条

[51] Enhanced ammonia-borane decomposition by synergistic catalysis using CoPd nanoparticles supported on titano-silicates [J].