Research progress on photocatalytic degradation of microplastics by graphitic carbon nitride

被引:1
作者
Zhang, Yuanbo [1 ]
Yu, Cailian [1 ,2 ]
Peng, Xianlong [3 ]
Yan, Hong [1 ]
Xu, Dan [1 ]
Lin, Yuchen [1 ]
机构
[1] Harbin Univ Sci & Technol, Coll Mat Sci & Chem Engn, Harbin 150080, Heilongjiang, Peoples R China
[2] Harbin Univ Sci & Technol, Coll Heilongjiang Prov, Sch Mat Sci & Chem Engn, Key Lab Green Chem Engn & Technol, Harbin 150080, Peoples R China
[3] Northeast Agr Univ, Coll Resources & Environm, Harbin 150038, Heilongjiang, Peoples R China
基金
中国国家自然科学基金;
关键词
Graphitic carbon nitride; Microplastic; Photocatalysis; Degradation mechanism; Factors affecting degradation; G-C3N4; LIGHT; TIO2; NANOMATERIALS; EFFICIENCY; WATER; PH; PHOTODEGRADATION; TRANSFORMATION; MICROSPHERES;
D O I
10.1007/s11164-024-05405-3
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
In recent years, the environmental problems caused by microplastics (MPs) as novel pollutants have received widespread attention, and photocatalytic technology can degrade MPs into small molecule compounds such as aldehydes and ketones. Among the existing catalysts, graphitic phase carbon nitride (g-C3N4) shows great potential in degrading pollutants due to its unique properties. In this paper, the structure, preparation method, modification method, mechanism of degradation of MPs and influencing factors of g-C3N4 are systematically reviewed. It is summarized that <middle dot>OH, h+, and <middle dot>O2- are the main active species in the degradation of MPs by g-C3N4, and the external conditions such as pH, light intensity, and the morphology of MPs themselves can affect the degradation of MPs. However, g-C3N4 photocatalytic degradation of MPs is still only in the laboratory stage at this stage, and problems such as the degradation of MPs in actual water bodies have not been carried out, so how to solve the above problems is the focus of future research in the field of g-C3N4 photocatalytic degradation of MPs.
引用
收藏
页码:5137 / 5165
页数:29
相关论文
共 94 条
[71]   Environment-friendly preparation of porous graphite-phase polymeric carbon nitride using calcium carbonate as templates, and enhanced photoelectrochemical activity [J].
Wang, Jianhai ;
Zhang, Cheng ;
Shen, Yanfei ;
Zhou, Zhixin ;
Yu, Jiachao ;
Li, Ying ;
Wei, Wei ;
Liu, Songqin ;
Zhang, Yuanjian .
JOURNAL OF MATERIALS CHEMISTRY A, 2015, 3 (09) :5126-5131
[72]   Oxygen defects-mediated Z-scheme charge separation in g-C3N4/ZnO photocatalysts for enhanced visible-light degradation of 4-chlorophenol and hydrogen evolution [J].
Wang, Jing ;
Xia, Yi ;
Zhao, Hongyuan ;
Wang, Guifang ;
Xiang, Lan ;
Xu, Jianlong ;
Komarneni, Sridhar .
APPLIED CATALYSIS B-ENVIRONMENTAL, 2017, 206 :406-416
[73]   Preparation of heterojunction C3N4/WO3 photocatalyst for degradation of microplastics in water [J].
Wang X. ;
Zhu Z. ;
Jiang J. ;
Li R. ;
Xiong J. .
Chemosphere, 2023, 337
[74]   Polymeric Graphitic Carbon Nitride for Heterogeneous Photocatalysis [J].
Wang, Xinchen ;
Blechert, Siegfried ;
Antonietti, Markus .
ACS CATALYSIS, 2012, 2 (08) :1596-1606
[75]  
Wang XC, 2009, NAT MATER, V8, P76, DOI [10.1038/nmat2317, 10.1038/NMAT2317]
[76]   Recent Advances on g-C3N4 Based Photocatalysts for Typical Antibiotics Photodegradation: Preparation, Mechanism and Influencing Factors [J].
Wang, Xuerong ;
Niu, Jinfen ;
Yang, Lan ;
Guo, Xingru ;
Yu, Xiaojiao ;
Yao, Binghua .
CHEMISTRYSELECT, 2023, 8 (47)
[77]   Polymeric Graphitic Carbon Nitride as a Heterogeneous Organocatalyst: From Photochemistry to Multipurpose Catalysis to Sustainable Chemistry [J].
Wang, Yong ;
Wang, Xinchen ;
Antonietti, Markus .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2012, 51 (01) :68-89
[78]   g-C3N4@α-Fe2O3/C Photocatalysts: Synergistically Intensified Charge Generation and Charge Transfer for NADH Regeneration [J].
Wu, Yizhou ;
Ward-Bond, Jesse ;
Li, Donglin ;
Zhang, Shaohua ;
Shi, Jiafu ;
Jiang, Zhongyi .
ACS CATALYSIS, 2018, 8 (07) :5664-5674
[79]   Photodegradation of Microplastics through Nanomaterials: Insights into Photocatalysts Modification and Detailed Mechanisms [J].
Xiao, Yiting ;
Tian, Yang ;
Xu, Wenbo ;
Zhu, Jun .
MATERIALS, 2024, 17 (11)
[80]   Photocatalytic Technologies for Transformation and Degradation of Microplastics in the Environment: Current Achievements and Future Prospects [J].
Xie, Anyou ;
Jin, Meiqing ;
Zhu, Jiangwei ;
Zhou, Qingwei ;
Fu, Li ;
Wu, Weihong .
CATALYSTS, 2023, 13 (05)