Flexible Single Microwire X-Ray Detector with Ultrahigh Sensitivity for Portable Radiation Detection System

被引:9
作者
Chen, Yancheng [1 ]
Niu, Shifeng [2 ]
Li, Ying [1 ]
Dou, Wenjie [3 ]
Yang, Xun [3 ]
Shan, Chongxin [3 ]
Shen, Guozhen [1 ]
机构
[1] Beijing Inst Technol, Sch Integrated Circuits & Elect, Beijing 100081, Peoples R China
[2] Henan Univ Sci & Technol, Sch Phys & Engn, Luoyang 471023, Peoples R China
[3] Zhengzhou Univ, Sch Phys & Microelect, Henan Key Lab Diamond Optoelect Mat & Devices, Key Lab Mat Phys,Minist Educ, Zhengzhou 450052, Peoples R China
基金
中国国家自然科学基金; 中国博士后科学基金;
关键词
flexible; Ga2O3; highly sensitive; portable radiation detection system; X-ray detector;
D O I
10.1002/adma.202404656
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Sensitive, flexible, and low false alarm rate X-ray detector is crucial for medical diagnosis, industrial inspection, and scientific research. However, most semiconductors for X-ray detectors are susceptible to interference from ambient light, and their high thickness hinders their application in wearable electronics. Herein, a flexible visible-blind and ultraviolet-blind X-ray detector based on Indium-doped Gallium oxide (Ga2O3:In) single microwire is prepared. Joint experiment-theory characterizations reveal that the Ga2O3:In microwire possess a high crystal quality, large band gap, and satisfactory stability, and reliability. On this basis, an extraordinary sensitivity of 5.9 x 10(5) mu C Gy(air)(-1) cm(-2) and a low detection limit of 67.4 nGy(air) s(-1) are achieved based on the prepared Ag/Ga2O3:In/Ag device, which has outstanding operation stability and excellent high temperature stability. Taking advantage of the flexible properties of the single microwire, a portable X-ray detection system is demonstrated that shows the potential to adapt to flexible and lightweight formats. The proposed X-ray detection system enables real-time monitor for X-rays, which can be displayed on the user interface. More importantly, it has excellent resistance to natural light interference, showing a low false alarm rate. This work provides a feasible method for exploring high-performance flexible integrated micro/nano X-ray detection devices.
引用
收藏
页数:10
相关论文
共 59 条
[1]  
Berger M. J., 2013, DATABASE NIST STANDA
[2]   Spatially nanoconfined N-type polymer semiconductors for stretchable ultrasensitive X-ray detection [J].
Bian, Yangshuang ;
Liu, Kai ;
Ran, Yang ;
Li, Yi ;
Gao, Yuanhong ;
Zhao, Zhiyuan ;
Shao, Mingchao ;
Liu, Yanwei ;
Kuang, Junhua ;
Zhu, Zhiheng ;
Qin, Mingcong ;
Pan, Zhichao ;
Zhu, Mingliang ;
Wang, Chenyu ;
Chen, Hu ;
Li, Jia ;
Li, Xifeng ;
Liu, Yunqi ;
Guo, Yunlong .
NATURE COMMUNICATIONS, 2022, 13 (01)
[3]   High Temperature Resistant Solar-Blind Ultraviolet Photosensor for Neuromorphic Computing and Cryptography [J].
Chen, Yancheng ;
Li, Ying ;
Niu, Shifeng ;
Yang, Xun ;
Dou, Wenjie ;
Shan, Chongxin ;
Shen, Guozhen .
ADVANCED FUNCTIONAL MATERIALS, 2024, 34 (24)
[4]   Ga2O3-Based Solar-Blind Position-Sensitive Detector for Noncontact Measurement and Optoelectronic Demodulation [J].
Chen, Yancheng ;
Yang, Xun ;
Zhang, Chongyang ;
He, Gaohang ;
Chen, Xuexia ;
Qiao, Qian ;
Zang, Jinhao ;
Dou, Wenjie ;
Sun, Pengxiang ;
Deng, Yuan ;
Dong, Lin ;
Shan, Chong-Xin .
NANO LETTERS, 2022, 22 (12) :4888-4896
[5]   Ultra-sensitive flexible Ga2O3 solar-blind photodetector array realized via ultra-thin absorbing medium [J].
Chen, Yancheng ;
Yang, Xun ;
Zhang, Yuan ;
Chen, Xuexia ;
Sun, Junlu ;
Xu, Zhiyang ;
Li, Kaiyong ;
Dong, Lin ;
Shan, Chongxin .
NANO RESEARCH, 2022, 15 (04) :3711-3719
[6]   Ultrasensitive and Robust CsPbBr3 Single-Crystal X-ray Detectors Based on Interface Engineering [J].
Chen, Zhilong ;
Wang, Hu ;
Li, Fenghua ;
Zhang, Wenqing ;
Shao, Yuchuan ;
Yang, Shuang .
ACS APPLIED MATERIALS & INTERFACES, 2023, 15 (44) :51370-51379
[7]   Lattice engineering for stabilized black FAPbI3 perovskite single crystals for high-resolution x-ray imaging at the lowest dose [J].
Chu, Depeng ;
Jia, Binxia ;
Liu, Naiming ;
Zhang, Yunxia ;
Li, Xiaotong ;
Feng, Jiangshan ;
Pi, Jiacheng ;
Yang, Zhou ;
Zhao, Guangtao ;
Liu, Yucheng ;
Liu, Shengzhong ;
Park, Nam-Gyu .
SCIENCE ADVANCES, 2023, 9 (35)
[8]   Perovskite-like Silver Halide Single-Crystal Microbelt Enables Ultrasensitive Flexible X-ray Detectors [J].
Dong, Kailian ;
Zhou, Hai ;
Shao, Wenlong ;
Gao, Zheng ;
Yao, Fang ;
Xiao, Meng ;
Li, Jiashuai ;
Liu, Yongjie ;
Wang, Shuxin ;
Zhou, Shun ;
Cui, Hongsen ;
Qin, Minchao ;
Lu, Xinhui ;
Tao, Chen ;
Ke, Weijun ;
Fang, Guojia .
ACS NANO, 2023, 17 (02) :1495-1504
[9]   Determination of the stability and magnetic properties of Fe-Pd nitride using the generalised gradient approximation (GGA) [J].
dos Santos, Antonio Vanderlei ;
Padilha, Gustavo ;
Moncalves, Matias .
SOLID STATE SCIENCES, 2012, 14 (02) :269-275
[10]   Atomically dispersed rhodium on ordered macroporous In2O3 for the highly sensitive detection of ethanol and the sensing mechanism [J].
Gu, Fubo ;
Zhang, Lanlan ;
Hong, Song ;
Han, Dongmei ;
Wang, Zhihua .
JOURNAL OF MATERIALS CHEMISTRY C, 2023, 11 (18) :5995-6003