Extended system-bath entanglement theorem with multiple baths in the presence of external fields

被引:0
|
作者
Qi, Hao-Yang [1 ]
Su, Yu [2 ,3 ]
Wang, Yao [2 ,3 ]
Xu, Rui-Xue [2 ,3 ]
Yan, Yijing [2 ]
机构
[1] Univ Sci & Technol China, Key Lab Precis & Intelligent Chem, Hefei 230026, Peoples R China
[2] Univ Sci & Technol China, Hefei Natl Res Ctr Phys Sci Microscale, Hefei 230026, Anhui, Peoples R China
[3] Univ Sci & Technol China, Hefei Natl Lab, Hefei 230088, Anhui, Peoples R China
来源
JOURNAL OF CHEMICAL PHYSICS | 2024年 / 161卷 / 12期
基金
中国国家自然科学基金;
关键词
QUANTUM; DYNAMICS; MOTION;
D O I
10.1063/5.0226351
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The system-bath entanglement theorem (SBET) was established in terms of linear response functions [Du et al., J. Chem. Phys. 152, 034102 (2020)] and generalized to correlation functions [Su et al., J. Chem. Phys. 160, 084104 (2024)] in our previous studies. This theorem connects the entangled system-bath properties to the local system and bare-bath ones. In this work, we extend the SBET to field-dressed conditions with multiple baths at different temperatures. As in reality, the external fields may interact with not only the system but also environments. The extended SBET facilitates, for example, photo-acoustic, photo-thermal, pump-probe related studies. The theorem under the field-free condition (multiple baths) and its counterpart in the classical limit is also presented.
引用
收藏
页数:9
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