2D Raman imaging for vibrational and rotational temperature mapping in H2

被引:0
作者
Del Cont-Bernard, D. [1 ]
Ruijzendaal, M. D. [1 ]
Righart, T. W. H. [1 ]
van Rooij, G. J. [1 ]
Butterworth, T. D. [1 ]
机构
[1] Maastricht Univ, Fac Sci & Engn, Dept Circular Chem Engn, POB 616, NL-6200 MD Maastricht, Netherlands
关键词
2D Raman scattering; Hydrogen; Hydrogen plasma; Interference bandpass filters; Thermometry; Vibrational-rotational non-equilibrium; FLAME; SCATTERING; NITROGEN;
D O I
10.1016/j.jqsrt.2024.109145
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
We showcase a Raman scattering diagnostic for 2D imaging of the rotational and vibrational temperatures of H2. 2 . Applications include environments with vibrational-rotational non-equilibrium such as H2 2-containing supersonic jets and plasma reactors. We image segments of the laser scattering spectrum, containing one or more Raman features, using an ICCD camera that is equipped with one of several bandpass filters. Knowing their transmission spectrum allows the construction of calibration curves that relate the relative intensities of the multi-spectral image to the rotational and vibrational temperatures. Additionally, the absolute intensity indicates the density of H2. 2 . We illustrate the capability to independently measure rotational (300-3000 K, +/- 150 K) and vibrational temperatures (1000-3000 K, +/- 50 K). The technique is demonstrated on two different H2 2 microwave plasmas and validated against conventional fitting of 0D and 1D Raman spectra.
引用
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页数:10
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共 34 条
  • [1] Ammonia as Effective Hydrogen Storage: A Review on Production, Storage and Utilization
    Aziz, Muhammad
    Wijayanta, Agung Tri
    Nandiyanto, Asep Bayu Dani
    [J]. ENERGIES, 2020, 13 (12)
  • [2] Communication: Two-dimensional gas-phase coherent anti-Stokes Raman spectroscopy (2D-CARS): Simultaneous planar imaging and multiplex spectroscopy in a single laser shot
    Bohlin, Alexis
    Kliewer, Christopher J.
    [J]. JOURNAL OF CHEMICAL PHYSICS, 2013, 138 (22)
  • [3] Plasma-driven dissociation of CO2 for fuel synthesis
    Bongers, Waldo
    Bouwmeester, Henny
    Wolf, Bram
    Peeters, Floran
    Welzel, Stefan
    van den Bekerom, Dirk
    den Harder, Niek
    Goede, Adelbert
    Graswinckel, Martijn
    Groen, Pieter Willem
    Kopecki, Jochen
    Leins, Martina
    van Rooij, Gerard
    Schulz, Andreas
    Walker, Matthias
    van de Sanden, Richard
    [J]. PLASMA PROCESSES AND POLYMERS, 2017, 14 (06)
  • [4] Two-dimensional Raman mole-fraction and temperature measurements for hydrogen-nitrogen mixture analysis
    Braeuer, Andreas
    Leipertz, Alfred
    [J]. APPLIED OPTICS, 2009, 48 (04) : B57 - B64
  • [5] Chen T, 2022, AIAA SCITECH 2022 forum, P2123, DOI [10.2514/6.2022-2123, DOI 10.2514/6.2022-2123]
  • [6] Numerical study of pure rotational fs/ps CARS coherence beating at high pressure and for multi-species rotation-vibration non-equilibrium thermometry
    Chen, Timothy Y.
    Kliewer, Christopher J.
    [J]. JOURNAL OF CHEMICAL PHYSICS, 2022, 157 (16)
  • [7] 1-D imaging of rotation-vibration non-equilibrium from pure rotational ultrafast coherent anti-Stokes Raman scattering
    Chen, Timothy Y.
    Goldberg, Benjamin M.
    Patterson, Brian D.
    Kolemen, Egemen
    Ju, Yiguang
    Kliewer, Christopher J.
    [J]. OPTICS LETTERS, 2020, 45 (15) : 4252 - 4255
  • [8] Cutler A, 2012, 28 AER MEAS TECHN GR, P3199, DOI [10.2514/6.2012-3199, DOI 10.2514/6.2012-3199]
  • [9] Dedic C., 2015, 46 AIAA PLASM LAS C, P2962, DOI [10.2514/6.2015-2962, DOI 10.2514/6.2015-2962]
  • [10] Single-shot ultrafast coherent anti-Stokes Raman scattering of vibrational/rotational nonequilibrium
    Dedic, Chloe E.
    Meyer, Terrence R.
    Michael, James B.
    [J]. OPTICA, 2017, 4 (05): : 563 - 570