Recent research progress of MOFs-based heterostructures for photocatalytic hydrogen evolution

被引:30
作者
Li, Jiaming [1 ,3 ]
Jia, Jia [2 ]
Wang, Deping [1 ]
Dong, Hongjun [1 ]
Zhu, Mingshan [4 ]
机构
[1] Jiangsu Univ, Inst Green Chem & Chem Technol, Sch Chem & Chem Engn, Zhenjiang 212013, Jiangsu, Peoples R China
[2] Baicheng Normal Univ, Baicheng 137000, Peoples R China
[3] Jilin Normal Univ, Coll Chem, Siping 136000, Peoples R China
[4] Jinan Univ, Sch Environm, Guangzhou 511443, Peoples R China
基金
中国国家自然科学基金;
关键词
Metal-organic frameworks; Heterostructure; Photocatalysis; H; 2; evolution; Reaction mechanism; METAL-ORGANIC FRAMEWORKS; FACILE CONSTRUCTION; WATER; HETEROJUNCTION; PERFORMANCE; CDS; NANOCOMPOSITES; FABRICATION; COMPOSITES; COCATALYST;
D O I
10.1016/j.cej.2024.155194
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The growing serious energy crisis and environmental pollution expedite the development of green hydrogen energy. Photocatalytic water splitting technology, converting solar energy into chemical energy directly, provides a clean and economical way for hydrogen evolution. For the past few years, metal-organic frameworks (MOFs) semiconductor materials have become a research hotspot in the field of photocatalytic hydrogen evolution (PHE) due to their multiple advantages, including adjustable structure, high porosity, large specific surface area, abundant active sites, and so forth. Besides this, the construction of heterogeneous structures based on MOFs materials can further improve PHE performance through the effective internal electric field directional transfer of photogenerated electrons and the superior utilization rate of sunlight in comparison to the single MOFs photocatalyst. Herein, in this minireview, we summed up the varieties of synthesis methods of diverse types of MOFs heterojunction complex materials, discussed the H2 evolution efficiency based on this heterostructure photocatalyst in detail, and lastly proposed the advantages, limitations, and outlook of MOFs composites in the PHE field. We sincerely hope this review can provide a reference for future research based on MOFs materials for alleviating the current energy crisis.
引用
收藏
页数:24
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