Ultrafast high harmonic generation in transition metal dichalcogenide quantum dots

被引:0
|
作者
Mitra, Aranyo [1 ]
Zafar, Ahmal Jawad [1 ]
Hosseini, Sayed Jaber [1 ]
Apalkov, Vadym [1 ]
机构
[1] Georgia State Univ, Dept Phys & Astron, Atlanta, GA 30303 USA
关键词
D O I
10.1103/PhysRevB.109.155425
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We study theoretically the generation of high harmonics by transition metal dichalcogenides disk-shaped quantum dots placed in an ultrashort optical pulse. The quantum dots are described within a massive Dirac type effective model with infinite mass boundary conditions. For a linearly polarized pulse, the cutoff frequency and the intensities of high-order harmonics increase with the quantum dot radius. For the frequency of the pulse below the system band gap, the radiation spectra show strong dependence on the quantum dot size, while for the large pulse frequency, i.e., above the band gap, both the intensities of high harmonics and cutoff frequency weakly depend on the quantum dot radius. For an elliptically polarized pulse, the intensities of harmonics monotonically decrease with the pulse ellipticity and become strongly suppressed for a circularly pulse. The cutoff frequency also monotonic decreases with the pulse ellipticity and shows weak dependence on the quantum dot material.
引用
收藏
页数:14
相关论文
共 50 条
  • [21] Second harmonic generation in nanoscale films of transition metal dichalcogenide: Accounting for multipath interference
    Kudryavtsev, A. V.
    Lavrov, S. D.
    Shestakova, A. P.
    Kulyuk, L. L.
    Mishina, E. D.
    AIP ADVANCES, 2016, 6 (09)
  • [22] Second Harmonic Generation from Artificially Stacked Transition Metal Dichalcogenide Twisted Bilayers
    Hsu, Wei-Ting
    Zhao, Zi-Ang
    Li, Lain-Jong
    Chen, Chang-Hsiao
    Chiu, Ming-Hui
    Chang, Pi-Shan
    Chou, Yi-Chia
    Chang, Wen-Hao
    ACS NANO, 2014, 8 (03) : 2951 - 2958
  • [23] Harmonic Generation by Metal Nanostructures Optically Coupled to Two-Dimensional Transition-Metal Dichalcogenide
    Drobnyh, Elena
    Pachter, Ruth
    Sukharev, Maxim
    JOURNAL OF PHYSICAL CHEMISTRY C, 2019, 123 (11): : 6898 - 6904
  • [24] High harmonic generation in graphene quantum dots with vacancy defects
    Gnawali, Suresh
    Apalkov, Vadym
    PHYSICA B-CONDENSED MATTER, 2025, 699
  • [25] Metallic Phase Transition Metal Dichalcogenide Quantum Dots as Promising Bio-Imaging Materials
    Park, Kwang Hyun
    Yang, Jun Yong
    Jung, Sunggyeong
    Ko, Byoung Min
    Song, Gian
    Hong, Soon-Jik
    Kim, Nam Chul
    Lee, Dongju
    Song, Sung Ho
    NANOMATERIALS, 2022, 12 (10)
  • [26] Controllable Interlayer Charge and Energy Transfer in Perovskite Quantum Dots/Transition Metal Dichalcogenide Heterostructures
    Liu, Huan
    Wang, Chong
    Wang, Ting
    Hu, Xiangmin
    Liu, Dameng
    Luo, Jianbin
    ADVANCED MATERIALS INTERFACES, 2019, 6 (23)
  • [27] Transition Metal Dichalcogenide Resonators for Second Harmonic Signal Enhancement
    Busschaert, Sebastian
    Reimann, Rene
    Cavigelli, Moritz
    Khelifa, Ronja
    Jain, Achint
    Novotny, Lukas
    ACS PHOTONICS, 2020, 7 (09): : 2482 - 2488
  • [28] Photocurrent generation in a metallic transition-metal dichalcogenide
    Mehmood, Naveed
    Rasouli, Hamid Reza
    Cakiroglu, Onur
    Kasirga, T. Serkan
    PHYSICAL REVIEW B, 2018, 97 (19)
  • [29] Ultrafast Dephasing and Coherent Exciton Dynamics in Transition Metal Dichalcogenide Bilayers
    Helmrich, Sophia
    Woggon, Ulrike
    Owschimikow, Nina
    Sampson, Kevin
    Tran, Kha
    Li, Xiaoqin
    2020 CONFERENCE ON LASERS AND ELECTRO-OPTICS (CLEO), 2020,
  • [30] Transition metal dichalcogenide quantum dots: Synthesis, properties, and applications for electrochemistry, energy storage, and solar cells
    Lee, Hoon Ju
    Yang, Weiguang
    Shin, Hyeon Suk
    BULLETIN OF THE KOREAN CHEMICAL SOCIETY, 2024, 45 (03) : 214 - 227