Laser-induced graphene: Carbon precursors, fabrication mechanisms, material characteristics, and applications in energy storage

被引:24
作者
Bai, Shigen [1 ]
Ruan, Luoyuan [1 ]
Chen, Huanjian [2 ]
Du, Yu [2 ]
Deng, Huiyong [3 ]
Dai, Ning [3 ,4 ,5 ]
Tang, Yong [6 ]
机构
[1] Zhejiang Lab, Res Ctr Frontier Fundamental Studies, Hangzhou 311100, Peoples R China
[2] Zhejiang Lab, Res Ctr Novel Computat Sensing & Intelligent Proc, Hangzhou 311100, Peoples R China
[3] Chinese Acad Sci, Shanghai Inst Tech Phys, State Key Lab Infrared Phys, Shanghai 200083, Peoples R China
[4] Univ Chinese Acad Sci, Hangzhou Inst Adv Study, Hangzhou 310024, Peoples R China
[5] Changzhou Univ, Jiangsu Collaborat Innovat Ctr Photovolta Sci & En, Changzhou 213164, Peoples R China
[6] South China Univ Technol, Sch Mech & Automot Engn, Guangzhou 510641, Peoples R China
基金
中国博士后科学基金; 中国国家自然科学基金;
关键词
Laser -induced graphene; Carbon precursor; Fabrication mechanism; Energy storage; Special surface area; Electrical conductivity; PHENOLIC RESIN; FUEL-CELL; PYROLYSIS MECHANISM; TG-FTIR; IN-SITU; PERFORMANCE; ELECTRODES; MICROSUPERCAPACITORS; AIR; NANOPARTICLES;
D O I
10.1016/j.cej.2024.152805
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Laser-induced graphene (LIG) has emerged as a highly promising electrode material for energy storage due to its exceptional physicochemical properties, including a well-developed 3D porosity structure, high specific surface area (SSA), excellent electrical conductivity (EC), impressive mechanical strength, and outstanding electrochemical stability. These merits are attributed to the localized transient high-temperature radiation and thermal expansion effects observed during laser processing. Extensive research efforts have been devoted to expanding carbon sources, investigating the formation mechanism of LIG, achieving controllable preparation of LIG and its composites with high SSA/EC, and exploring their applications in energy storage and other domains. This review provides a comprehensive account of LIG, starting with an overview of the mainstream carbon precursors: polymer substrates, phenolic resins, and lignocellulosic materials. Subsequently, the fabrication mechanisms for transforming these carbon source matrices into 3D porous graphene are thoroughly examined. Additionally, the unique advantages of LIG and its composites are summarized, encompassing controllable surface micromorphology, high SSA and EC, efficient wetting properties with full contact angle coverage, and superior mechanical flexibility. Furthermore, the review presents an extensive survey of the applications of LIG and its doped, modified, or multi-composite materials in planar flexible supercapacitors, various battery systems (such as lithium-ion, sodium-ion, lithium-metal, metal-air, and lithium-sulfur batteries), as well as fuel cells (including bio-, chemical, microfluidic, alumina-air, and proton exchange membrane fuel cells). Finally, the review concludes with an outlook on future challenges and perspectives in the research and development of LIG materials and their associated devices in the field of energy storage.
引用
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页数:23
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