Updating vehicle VOCs emissions characteristics under clean air actions in a tropical city of China

被引:1
作者
Huo, Sisi [1 ]
Zhang, Xin [1 ]
Xu, Wenshuai [3 ,4 ]
Dang, Juan [1 ]
Xu, Fei [1 ]
Xie, Wenjing [2 ,3 ]
Tao, Chenliang [1 ]
Han, Yanan [1 ]
Liu, Xinning [1 ]
Teng, Zhuochao [1 ]
Xie, Rongfu [2 ,3 ]
Cao, Xiaocong [2 ,3 ]
Zhang, Qingzhu [1 ]
机构
[1] Shandong Univ, Environm Res Inst, Qingdao 266237, Peoples R China
[2] Peking Univ, Coll Environm Sci & Engn, State Key Joint Lab Environm Simulat & Pollut Cont, Beijing 100871, Peoples R China
[3] Hainan Res Acad Environm Sci, Haikou 571126, Peoples R China
[4] Hainan Prov Ecol & Environm Monitoring Ctr, Haikou 571126, Peoples R China
关键词
Vehicle emissions; VOCs; Emission factors; Clean air actions; Tunnel experiments; VOLATILE ORGANIC-COMPOUNDS; ON-ROAD VEHICLES; EVAPORATIVE EMISSIONS; URBAN TUNNEL; IMPACTS; ELECTRIFICATION; QUALITY;
D O I
10.1016/j.scitotenv.2024.172733
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
In the context of clean air actions in China, vehicle emission limits have been continuously tightened, which has facilitated the reduction of volatile organic compounds (VOCs) emissions. However, the characteristics of VOC emissions from vehicles with strict emission limits are poorly understood. This study investigated the VOC emission characteristics from vehicles under the latest standards based on tunnel measurements, and identified future control strategies for vehicle emissions. The results showed that the highest percentage of VOCs from vehicle consisted of alkanes (80.9 %), followed by aromatics (15.8 %) and alkenes (3.1 %). Alkanes had the most significant ozone formation potential due to their high concentrations, in contrast to the aromatics that have been dominant in previous studies. The measured fleet-average VOC emission factor was 71.3 mg & sdot;km- 1, including tailpipe emissions of 39.6 mg & sdot;km- 1 and evaporative emissions of 31.7 mg & sdot;km- 1. The VOC emission factors of the subgroups were obtained. The emission of evaporated VOCs accounted for 44.5 % of the total vehicle VOC emissions, which have increased substantially from previous studies. In addition, the emission characteristics of vehicles that are under the latest emission threshold values have changed significantly, and the mixing ratio of toluene/benzene (T/B) has been updated to 3:1. This study updates the VOCs emission factors of vehicles under clean air actions and highlights the future mitigation policies should focus on reducing evaporative VOC emissions.
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页数:11
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