The performance and applicability study of a photovoltaic-driven electro-Fenton wastewater treatment system

被引:5
作者
Zeng, Xiding [1 ,2 ]
Zhang, Wei [1 ,2 ]
Zhang, Jing [1 ,2 ]
Liang, Juan [1 ]
Xie, Lingzhi [3 ]
Guo, Jiahong [1 ,2 ]
Zhong, Jianmei [1 ,2 ]
Li, Zhangyu [1 ,2 ]
Yang, Kun [1 ,2 ]
Zhang, Chenyang [1 ,2 ]
Wang, Qing [1 ,2 ]
机构
[1] Sichuan Univ, Coll Architecture & Environm, Chengdu 610065, Peoples R China
[2] Sichuan Univ, Yibin Ind Technol Res Inst, Yibin 644000, Peoples R China
[3] Sichuan Univ, Inst New Energy & Low Carbon Technol, Chengdu 610065, Peoples R China
关键词
Wastewater treatment; Photovoltaics; Electro-Fenton; Degradation efficiency; SOLAR PHOTO-FENTON; TREATMENT PLANTS; DEGRADATION; REMOVAL; RECOVERY;
D O I
10.1016/j.enconman.2024.118617
中图分类号
O414.1 [热力学];
学科分类号
摘要
In the current mainstream wastewater treatment technologies, electro-Fenton (EF) has been widely used as an advanced oxidation process for achieving deep degradation of organic pollutants without secondary pollution. However, the high energy consumption of EF has hindered its development to a certain extent. In this study, a photovoltaic(PV)-driven EF system is developed to incorporate photovoltaic energy into the EF system to efficiently degrade organic matter in sewage and reduce energy consumption and operating costs of sewage treatment. To fully evaluate the performance of the photovoltaic drive electro-Fenton degradation sewage (PVEF) system, we investigated the effects of system configuration, current density, and stirring speed on the degradation of methyl orange (AO7) by the PVEF system. After determining the optimal experimental conditions, we explored the treatment efficiency and feasibility of the system for three different types of pollutants. Laboratory scale experiments also confirmed the critical effects of current density and stirring speed on the energy consumption of degradation. Finally, PVEF technology replaces the advanced treatment process in the sewage treatment plant, and the energy consumption model is established based on the local dye sewage plant in Chengdu to evaluate its applicability in different regions. The experimental results show that the dual-cathode system reduced energy consumption by 24.9 % and increased degradation efficiency by 30 % compared to the conventional EF system & sdot;H 2 O 2 generated under the optimal conditions is fully utilized, resulting in a removal rate of more than 95 % in 20 min for AO7. The optimal energy efficiency condition is determined when the current density is 3 mA/cm 2 and the stirring speed is 1000 rpm, which reduces the system 's energy consumption. The degradation test results of different pollutants show that the system can realize the degradation of various pollutants. The simulation results of the sewage plant scale show that the PVEF system can reduce carbon emission by 305 t instead of the traditional advanced treatment process.
引用
收藏
页数:12
相关论文
共 41 条
[1]  
Campana PE, 2021, Energy Convers Manage, P239
[2]   Energy Issues in Sustainable Urban Wastewater Management: Use, Demand Reduction and Recovery in the Urban Water Cycle [J].
Capodaglio, Andrea G. ;
Olsson, Gustaf .
SUSTAINABILITY, 2020, 12 (01)
[3]   Reliable energy recovery in an existing municipal wastewater treatment plant with a flow-variable micro-hydropower system [J].
Chae, Kyu-Jung ;
Kim, In-Soo ;
Ren, Xianghao ;
Cheon, Kyeong-Ho .
ENERGY CONVERSION AND MANAGEMENT, 2015, 101 :681-688
[4]   Boron Bifunctional Catalysts for Rapid Degradation of Persistent Organic Pollutants in a Metal-Free Electro-Fenton Process: O2 and H2O2 Activation Process [J].
Chen, Xu ;
Wang, Lida ;
Sun, Wen ;
Yang, Zhengqing ;
Jin, Jingjing ;
Huang, YaPeng ;
Liu, Guichang .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2023, 57 (41) :15693-15702
[5]  
Cui LL, 2023, GREEN CHEM, V25, P6315, DOI [10.1039/d3gc01653f, 10.1039/D3GC01653F]
[6]   Enhancement of a solar photo-Fenton reaction by using ferrioxalate complexes for the treatment of a synthetic cotton-textile dyeing wastewater [J].
Doumic, Lucila I. ;
Soares, Petrick A. ;
Ayude, Maria A. ;
Cassanello, Miryan ;
Boaventura, Rui A. R. ;
Vilar, Vitor J. P. .
CHEMICAL ENGINEERING JOURNAL, 2015, 277 :86-96
[7]   Decolorizing textile wastewater with Fenton's reagent electrogenerated with a solar photovoltaic cell [J].
Figueroa, Sandra ;
Vazquez, Leticia ;
Alvarez-Gallegos, A. .
WATER RESEARCH, 2009, 43 (02) :283-294
[8]   Carbon reduction measures-based life cycle assessment of the photovoltaic-supported sewage treatment system [J].
Guo, Jiahong ;
Zhang, Wei ;
Zhang, Jing ;
Xie, Lingzhi ;
Zeng, Xiding ;
Zhong, Jianmei ;
Zhao, Oufan ;
Yang, Kun ;
Li, Zhangyu ;
Zou, Ruiwen ;
Bai, Zepu ;
Wang, Qing ;
Zhang, Chenyang .
SUSTAINABLE CITIES AND SOCIETY, 2024, 101
[9]  
Guo X, 2021, Appl Surf Sci, P556
[10]   The experimental study of a hybrid solar photo-Fenton and photovoltaic system for water purification [J].
Jin, Yanchao ;
Wang, Yiping ;
Huang, Qunwu ;
Zhu, Li ;
Cui, Yong ;
Cui, Lingyun ;
Lin, Chunyan .
ENERGY CONVERSION AND MANAGEMENT, 2017, 135 :178-187