Photomolecular effect: Visible light interaction with air-water interface

被引:12
|
作者
Lv, Guangxin [1 ]
Tu, Yaodong [1 ]
Zhang, James H. [1 ]
机构
[1] MIT, Dept Mech Engn, Cambridge, MA 02139 USA
关键词
photomolecular effect; water clusters; superthermal evaporation; cloud absorption; solar interfacial evaporation; MOLECULAR-DYNAMICS; SOLAR-RADIATION; LIQUID; CLOUDS; VAPOR; SPECTROSCOPY; ABSORPTION; CLUSTERS;
D O I
10.1073/pnas.2320844121
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Although water is almost transparent to visible light, we demonstrate that the air-water interface interacts strongly with visible light via what we hypothesize as the photomolecular effect. In this effect, transverse - magnetic polarized photons cleave off water clusters from the air-water interface. We use 14 different experiments to demonstrate the existence of this effect and its dependence on the wavelength, incident angle, and polarization of visible light. We further demonstrate that visible light heats up thin fogs, suggesting that this process can impact weather, climate, and the earth's water cycle and that it provides a mechanism to resolve the long - standing puzzle of larger measured clouds absorption to solar radiation than theory could predict based on bulk water optical constants. Our study suggests that the photomolecular effect should happen widely in nature, from clouds to fogs, ocean to soil surfaces, and plant transpiration and can also lead to applications in energy and clean water.
引用
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页数:9
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