Preparation of colored TiO 2 flower/Ti 3 C 2 for efficient photocatalytic degradation of tetracycline

被引:6
|
作者
Deng, Quanhao [1 ,2 ]
Yu, Leyang [1 ,2 ]
Chen, Qianmei [1 ,2 ]
Wen, Jianfeng [1 ,2 ]
Zhang, Anqi [1 ,2 ]
Li, Ming [1 ,2 ]
Tang, Tao [1 ,2 ]
Hu, Guanghui [1 ,2 ]
Jiang, Li [1 ,2 ]
Cao, Xueli [1 ,2 ]
Yao, Yi [2 ,3 ]
机构
[1] Guilin Univ Technol, Coll Phys & Elect Informat Engn, Guilin 541004, Peoples R China
[2] Guilin Univ Technol, Educ Dept Guangxi Zhuang Autonomous Reg, Key Lab Low dimens Struct Phys & Applicat, Guilin 541004, Peoples R China
[3] Guilin Univ Technol, Coll Environm Sci & Engn, Guangxi Collaborat Innovat Ctr Water Pollut Contro, 319 Yanshan St, Guilin 541004, Peoples R China
关键词
ColoredTiO2; Oxygen vacancy; Photocatalysis; NaHB4; STEP HYDROTHERMAL SYNTHESIS; VISIBLE-LIGHT; HYDROGEN-PRODUCTION; CHARGE-TRANSFER; DOPED TIO2; WATER; ANTIBIOTICS; NANOCOMPOSITE; OXIDATION; COMPOSITE;
D O I
10.1016/j.inoche.2024.112317
中图分类号
O61 [无机化学];
学科分类号
070301 ; 081704 ;
摘要
Herein, colored TiO 2 flowers grown on Ti 3 C 2 (XTFT, where X = 250 degrees C, 300 degrees C, and 350 degrees C representing heating temperature) are prepared as photocatalysts for degradation of tetracycline using hydrothermal method and CVD process. TiO 2 has a suitable bandgap as a photocatalyst. However, in practical applications, TiO 2 cannot effectively utilize visible light and the recombination of photogenerated carriers is excessively fast. The fabrication of XTFT through defect engineering compensates for the shortcomings of pure TiO 2 in photocatalytic applications, following which the bandgap of TiO 2 is reduced and the TiO 2 surface becomes discolored and effectively responds to visible light. Ti 3 C 2 , a promising auxiliary material in the field of photocatalysis, is used as a photocatalyst in the degradation of tetracycline via defect engineering. After forming a composite with TiO 2 , Ti 3 C 2 can effectively separate TiO 2 photogenerated carriers to enhance the photocatalytic performance of TiO 2 . The degradation rate of 50 mL 50 mg/L tetracycline by 50 mg 300TFT under visible light irradiation for 30 min is 96.3 %. Compared with pure TiO 2 , the photocatalytic efficiency is significantly improved, thus providing a new idea for realization of highly efficient visible photocatalysis in the field of environmental pollution in future.
引用
收藏
页数:10
相关论文
共 50 条
  • [31] Preparation of g-C3N4/TiO2 Nanocomposites and Investigation of Their Photocatalytic Activity
    Li, Qiuye
    Zong, Lanlan
    Xing, Yangyang
    Wang, Xiaodong
    Yu, Laigui
    Yang, Jianjun
    SCIENCE OF ADVANCED MATERIALS, 2013, 5 (09) : 1316 - 1322
  • [32] Compact and uniform TiO2@g-C3N4 core-shell quantum heterojunction for photocatalytic degradation of tetracycline antibiotics
    Wang, Wei
    Fang, Jiaojiao
    Shao, Shaofeng
    Lai, Min
    Lu, Chunhua
    APPLIED CATALYSIS B-ENVIRONMENTAL, 2017, 217 : 57 - 64
  • [33] Modification of g-C3N4 Photocatalyst with Flower-like ReS2 for Highly Efficient Photocatalytic Hydrogen Evolution
    Xing, Chuanwang
    Zhao, Haitao
    Yu, Guiyang
    Guo, Luyan
    Hu, Yujia
    Chen, Ting
    Jiang, Lilin
    Li, Xiyou
    CHEMCATCHEM, 2020, 12 (24) : 6385 - 6392
  • [34] Synthesis of C/N-TiO2@MIL-100(Fe) for highly efficient photocatalytic degradation of tetracycline under visible light irradiation
    Cao, Fazhao
    You, Mengqin
    Huang, Linchuan
    Zhu, Chenfei
    Liao, Hang
    Du, Jun
    JOURNAL OF PHOTOCHEMISTRY AND PHOTOBIOLOGY A-CHEMISTRY, 2024, 451
  • [35] Efficient degradation of tetracycline hydrochloride by photocatalytic ozonation over Bi2WO6
    Lu, Tong
    Gao, Yan
    Yang, Yang
    Ming, Hongbo
    Huang, Zhongcheng
    Liu, Guodong
    Zheng, DanDan
    Zhang, Jinshui
    Hou, Yidong
    CHEMOSPHERE, 2021, 283
  • [36] Preparation of α-Fe2O3-TiO2/fly ash cenospheres photocatalyst and its mechanism of photocatalytic degradation
    Liu, Shaomin
    Zhu, Jinglin
    Guo, Xuetao
    Ge, Jianhua
    Wu, Huijun
    COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS, 2015, 484 : 434 - 440
  • [37] Preparation and Characterization of Sb2S3-TiO2 Nanocomposite for the Enhanced Photocatalytic Degradation and Mineralization of Azo Dye
    Shitole, Kirti D.
    Patil, Anagha B.
    Thakur, Pragati
    ENVIRONMENTAL ENGINEERING SCIENCE, 2016, 33 (08) : 536 - 543
  • [38] TiO2/Ti3C2Tx gel microsphere for efficient photocatalytic degradation of organic pollutant with excellent recycling stability
    Wang, Dan
    Yang, Yan
    Chen, Yinxiang
    Yao, Chen
    Zhang, Zhijun
    Zhang, Ye
    JOURNAL OF WATER PROCESS ENGINEERING, 2024, 66
  • [39] Solar light efficient photocatalytic activity degradation of emergent contaminants by coated TiO2 nanoparticles
    Emilia Villanueva, Maria
    Javier Copello, Guillermo
    Campo Dall'Orto, Viviana
    NEW JOURNAL OF CHEMISTRY, 2018, 42 (18) : 15405 - 15412
  • [40] An Efficient, Multi-element AC/TiO2/WO3 Photocatalyst for the Degradation of Tetracycline Hydrochloride
    Xu, Mengdi
    Nan, Hui
    Yang, Hao
    Xue, Caihong
    Fu, Hua
    Yang, Guijun
    Chen, Huiyuan
    Lin, Hong
    CHEMISTRYSELECT, 2022, 7 (08):