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Preparation of colored TiO 2 flower/Ti 3 C 2 for efficient photocatalytic degradation of tetracycline
被引:6
|作者:
Deng, Quanhao
[1
,2
]
Yu, Leyang
[1
,2
]
Chen, Qianmei
[1
,2
]
Wen, Jianfeng
[1
,2
]
Zhang, Anqi
[1
,2
]
Li, Ming
[1
,2
]
Tang, Tao
[1
,2
]
Hu, Guanghui
[1
,2
]
Jiang, Li
[1
,2
]
Cao, Xueli
[1
,2
]
Yao, Yi
[2
,3
]
机构:
[1] Guilin Univ Technol, Coll Phys & Elect Informat Engn, Guilin 541004, Peoples R China
[2] Guilin Univ Technol, Educ Dept Guangxi Zhuang Autonomous Reg, Key Lab Low dimens Struct Phys & Applicat, Guilin 541004, Peoples R China
[3] Guilin Univ Technol, Coll Environm Sci & Engn, Guangxi Collaborat Innovat Ctr Water Pollut Contro, 319 Yanshan St, Guilin 541004, Peoples R China
关键词:
ColoredTiO2;
Oxygen vacancy;
Photocatalysis;
NaHB4;
STEP HYDROTHERMAL SYNTHESIS;
VISIBLE-LIGHT;
HYDROGEN-PRODUCTION;
CHARGE-TRANSFER;
DOPED TIO2;
WATER;
ANTIBIOTICS;
NANOCOMPOSITE;
OXIDATION;
COMPOSITE;
D O I:
10.1016/j.inoche.2024.112317
中图分类号:
O61 [无机化学];
学科分类号:
070301 ;
081704 ;
摘要:
Herein, colored TiO 2 flowers grown on Ti 3 C 2 (XTFT, where X = 250 degrees C, 300 degrees C, and 350 degrees C representing heating temperature) are prepared as photocatalysts for degradation of tetracycline using hydrothermal method and CVD process. TiO 2 has a suitable bandgap as a photocatalyst. However, in practical applications, TiO 2 cannot effectively utilize visible light and the recombination of photogenerated carriers is excessively fast. The fabrication of XTFT through defect engineering compensates for the shortcomings of pure TiO 2 in photocatalytic applications, following which the bandgap of TiO 2 is reduced and the TiO 2 surface becomes discolored and effectively responds to visible light. Ti 3 C 2 , a promising auxiliary material in the field of photocatalysis, is used as a photocatalyst in the degradation of tetracycline via defect engineering. After forming a composite with TiO 2 , Ti 3 C 2 can effectively separate TiO 2 photogenerated carriers to enhance the photocatalytic performance of TiO 2 . The degradation rate of 50 mL 50 mg/L tetracycline by 50 mg 300TFT under visible light irradiation for 30 min is 96.3 %. Compared with pure TiO 2 , the photocatalytic efficiency is significantly improved, thus providing a new idea for realization of highly efficient visible photocatalysis in the field of environmental pollution in future.
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页数:10
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