Amyloid Proteins Adhesive for Slippery Liquid-Infused Porous Surfaces

被引:0
|
作者
Feng, Na [1 ]
Miao, Shuting [2 ]
Guo, Xin [2 ]
Yang, Ziyi [2 ]
Yan, Luke [2 ]
Yang, Peng [2 ,3 ,4 ]
Kong, Jia [2 ]
机构
[1] Changan Univ, Sch Mat Sci & Engn, Xian 710072, Peoples R China
[2] Shaanxi Normal Univ, Sch Chem & Chem Engn, Key Lab Appl Surface & Colloid Chem, Minist Educ, Xian 710119, Peoples R China
[3] Shaanxi Normal Univ, Sch Chem & Chem Engn, Xian Key Lab Polymer Soft Matter, Xian 710119, Peoples R China
[4] Shaanxi Normal Univ, Int Joint Res Ctr Funct Fiber & Soft Smart Text, Sch Chem & Chem Engn, Xian 710119, Peoples R China
基金
国家重点研发计划; 中国博士后科学基金; 中国国家自然科学基金;
关键词
amyloid protein; anti-corrosion; anti-fouling; anti-icing; slippery liquid-infused porous surfaces; ROBUST;
D O I
10.1002/marc.202400596
中图分类号
O63 [高分子化学(高聚物)];
学科分类号
070305 ; 080501 ; 081704 ;
摘要
Biomimetic slippery liquid-infused porous surfaces (SLIPS) have emerged as a promising solution to solve the limitations of superhydrophobic surfaces, such as inadequate durability in corrosion protection and a propensity for frosting. However, the challenge of ensuring strong, lasting adhesion on diverse materials to enhance the durability of the lubricant layer remains. The research addresses this by leveraging amyloid phase-transitioned lysozyme (PTL) as an adhesive interlayer, conferring stable attachment of SLIPS across a variety of substrates, including metals, inorganics, and polymers. The silica-textured interface robustly secures the lubricant with a notably low sliding angle of 1.15 degrees. PTL-mediated adhesion fortifies the silicone oil attachment to the substrate, ensuring the retention of its repellent efficacy amidst mechanical stressors like ultrasonication, water scrubbing, and centrifugation. The integration of robust adhesion, cross-substrate compatibility, and durability under stress affords the PTL-modified SLIPS exceptional anti-fouling, anti-icing, and anti-corrosion properties, marking it as a leading solution for advanced protective applications. The utilization of amyloid phase-transitioned lysozyme (PTL) as an adhesive interlayer enhances the biosafety, transparency, and stability of SLIPS on diverse substrates. The incorporation of strong adhesion, compatibility across substrates, and resilience to stress endows PTL-modified SLIPS with outstanding anti-fouling, anti-icing, and anti-corrosion properties, positioning it as a top-tier solution for advanced protective applications. image
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页数:8
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