Sum-frequency generation from chiral bulk media holds the promise of a powerful tool in the investigation of biological as well as artificial materials containing optically active elements. Since this technique is based on a nonlinear optical effect, the high intensities of the illuminating light sources may induce spurious artifacts. Using simple conjugated chromophores, we demonstrate that multi-photon induced irreversible photolysis may be avoided while keeping undiminished levels of sum-frequency signals. In addition we show that the concurrent multi-photon induced luminescence may provide complementary means of imaging samples. (C) 2015 Published by Elsevier B.V.
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Fritz Haber Inst Max Planck Gesellschaft, Faradayweg 4-6, D-14195 Berlin, GermanyFritz Haber Inst Max Planck Gesellschaft, Faradayweg 4-6, D-14195 Berlin, Germany
Niemann, Richarda
Mueller, Niclas S.
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Fritz Haber Inst Max Planck Gesellschaft, Faradayweg 4-6, D-14195 Berlin, GermanyFritz Haber Inst Max Planck Gesellschaft, Faradayweg 4-6, D-14195 Berlin, Germany
Mueller, Niclas S.
Wasserroth, Soeren
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Fritz Haber Inst Max Planck Gesellschaft, Faradayweg 4-6, D-14195 Berlin, GermanyFritz Haber Inst Max Planck Gesellschaft, Faradayweg 4-6, D-14195 Berlin, Germany
Wasserroth, Soeren
Lu, Guanyu
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Vanderbilt Univ, Dept Mech Engn, Nashville, TN 37235 USA
Northwestern Univ, Dept Chem & Biol Engn, 2145 Sheridan Rd, Evanston, IL 60208 USAFritz Haber Inst Max Planck Gesellschaft, Faradayweg 4-6, D-14195 Berlin, Germany
Lu, Guanyu
Wolf, Martin
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Fritz Haber Inst Max Planck Gesellschaft, Faradayweg 4-6, D-14195 Berlin, GermanyFritz Haber Inst Max Planck Gesellschaft, Faradayweg 4-6, D-14195 Berlin, Germany
Wolf, Martin
Caldwell, Joshua D.
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Vanderbilt Univ, Dept Mech Engn, Nashville, TN 37235 USA
Vanderbilt Univ, Interdisciplinary Mat Sci Grad Program, Nashville, TN 37235 USAFritz Haber Inst Max Planck Gesellschaft, Faradayweg 4-6, D-14195 Berlin, Germany
Caldwell, Joshua D.
Paarmann, Alexander
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Fritz Haber Inst Max Planck Gesellschaft, Faradayweg 4-6, D-14195 Berlin, GermanyFritz Haber Inst Max Planck Gesellschaft, Faradayweg 4-6, D-14195 Berlin, Germany
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Univ New South Wales, Sch Photovolta & Renewable Energy Engn, Sydney, NSW 2052, AustraliaUniv New South Wales, Sch Photovolta & Renewable Energy Engn, Sydney, NSW 2052, Australia
Upama, Mushfika Baishakhi
Elumalai, Naveen Kumar
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Univ New South Wales, Sch Photovolta & Renewable Energy Engn, Sydney, NSW 2052, AustraliaUniv New South Wales, Sch Photovolta & Renewable Energy Engn, Sydney, NSW 2052, Australia
Elumalai, Naveen Kumar
Mahmud, Md Arafat
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Univ New South Wales, Sch Photovolta & Renewable Energy Engn, Sydney, NSW 2052, AustraliaUniv New South Wales, Sch Photovolta & Renewable Energy Engn, Sydney, NSW 2052, Australia
Mahmud, Md Arafat
Sun, Heng
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Univ New South Wales, Sch Photovolta & Renewable Energy Engn, Sydney, NSW 2052, AustraliaUniv New South Wales, Sch Photovolta & Renewable Energy Engn, Sydney, NSW 2052, Australia
Sun, Heng
Wang, Dian
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Univ New South Wales, Sch Photovolta & Renewable Energy Engn, Sydney, NSW 2052, AustraliaUniv New South Wales, Sch Photovolta & Renewable Energy Engn, Sydney, NSW 2052, Australia
Wang, Dian
Chan, Kah Howe
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Univ New South Wales, Sch Photovolta & Renewable Energy Engn, Sydney, NSW 2052, AustraliaUniv New South Wales, Sch Photovolta & Renewable Energy Engn, Sydney, NSW 2052, Australia
Chan, Kah Howe
Wright, Matthew
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Univ New South Wales, Sch Photovolta & Renewable Energy Engn, Sydney, NSW 2052, AustraliaUniv New South Wales, Sch Photovolta & Renewable Energy Engn, Sydney, NSW 2052, Australia
Wright, Matthew
Xu, Cheng
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Univ New South Wales, Sch Photovolta & Renewable Energy Engn, Sydney, NSW 2052, AustraliaUniv New South Wales, Sch Photovolta & Renewable Energy Engn, Sydney, NSW 2052, Australia
Xu, Cheng
Uddin, Ashraf
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Univ New South Wales, Sch Photovolta & Renewable Energy Engn, Sydney, NSW 2052, AustraliaUniv New South Wales, Sch Photovolta & Renewable Energy Engn, Sydney, NSW 2052, Australia
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Max Planck Gesell, Fritz Haber Inst, Faradayweg 4-6, D-14195 Berlin, GermanyMax Planck Gesell, Fritz Haber Inst, Faradayweg 4-6, D-14195 Berlin, Germany
Kiessling, Riko
Tong, Yujin
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Max Planck Gesell, Fritz Haber Inst, Faradayweg 4-6, D-14195 Berlin, GermanyMax Planck Gesell, Fritz Haber Inst, Faradayweg 4-6, D-14195 Berlin, Germany
Tong, Yujin
Giles, Alexander J.
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US Naval Res Lab, 4555 Overlook Ave SW, Washington, DC 20375 USAMax Planck Gesell, Fritz Haber Inst, Faradayweg 4-6, D-14195 Berlin, Germany
Giles, Alexander J.
Gewinner, Sandy
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Max Planck Gesell, Fritz Haber Inst, Faradayweg 4-6, D-14195 Berlin, GermanyMax Planck Gesell, Fritz Haber Inst, Faradayweg 4-6, D-14195 Berlin, Germany
Gewinner, Sandy
Schoellkopf, Wieland
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Max Planck Gesell, Fritz Haber Inst, Faradayweg 4-6, D-14195 Berlin, GermanyMax Planck Gesell, Fritz Haber Inst, Faradayweg 4-6, D-14195 Berlin, Germany
Schoellkopf, Wieland
Caldwell, Joshua D.
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US Naval Res Lab, 4555 Overlook Ave SW, Washington, DC 20375 USA
Vanderbilt Univ, Dept Mech Engn, 2400 Highland Ave, Nashville, TN 37212 USAMax Planck Gesell, Fritz Haber Inst, Faradayweg 4-6, D-14195 Berlin, Germany
Caldwell, Joshua D.
Wolf, Martin
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Max Planck Gesell, Fritz Haber Inst, Faradayweg 4-6, D-14195 Berlin, GermanyMax Planck Gesell, Fritz Haber Inst, Faradayweg 4-6, D-14195 Berlin, Germany
Wolf, Martin
Paarmann, Alexander
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Max Planck Gesell, Fritz Haber Inst, Faradayweg 4-6, D-14195 Berlin, GermanyMax Planck Gesell, Fritz Haber Inst, Faradayweg 4-6, D-14195 Berlin, Germany
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Natl Inst Adv Ind Sci & Technol, Nanosyst Res Inst, Tsukuba, Ibaraki 3058565, Japan
Chem Mat Evaluat & Res Base CEREBA, Tsukuba, Ibaraki 3050053, JapanNatl Inst Adv Ind Sci & Technol, Nanosyst Res Inst, Tsukuba, Ibaraki 3058565, Japan
Miyamae, T.
Takada, N.
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Chem Mat Evaluat & Res Base CEREBA, Tsukuba, Ibaraki 3050053, Japan
Natl Inst Adv Ind Sci & Technol, Flexible Elect Res Ctr, Tsukuba, Ibaraki 3058565, JapanNatl Inst Adv Ind Sci & Technol, Nanosyst Res Inst, Tsukuba, Ibaraki 3058565, Japan
Takada, N.
Tautsui, T.
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Chem Mat Evaluat & Res Base CEREBA, Tsukuba, Ibaraki 3050053, JapanNatl Inst Adv Ind Sci & Technol, Nanosyst Res Inst, Tsukuba, Ibaraki 3058565, Japan