The integrated approach of carbon capture, utilization, and storage via CO2 mineralization for the removal of fly ash, bottom ash, and exhaust gas-A case study of circulating fluidized bed combustion

被引:4
作者
Jeong, Eunhoo [1 ]
Jung, Seok-Ho [2 ]
Shin, Hyun-Sang [1 ]
机构
[1] Seoul Natl Univ Sci & Technol, Dept Environm Engn, Seoul 01811, South Korea
[2] Healthcare & Spa Ind Promot Agcy, Dept Corp Support, Asan 31442, South Korea
关键词
Bottom ash; Fly ash; CCUS; CFBC; CO; 2; mineralization; FIRED POWER-PLANTS; COAL; SEQUESTRATION; CEMENT; ISSUES; SCALE; RATIO;
D O I
10.1016/j.scitotenv.2024.174104
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Despite efforts to reduce dependence on coal-fired power generation due to climate concerns, continued usage for energy stability is anticipated. This study was conducted to address environmental issues associated with coal-fired power generation and promote its persistent utilization. we aimed to establish both eco-friendly and economically sustainable practices by mitigating waste such as fly ash (FA) and bottom ash (BA) emissions while recycling them in circulating fluidized bed combustion (CFBC). Initially, we conducted a literature review to analyze the global and domestic trends in coal-fired power generation. Subsequently, we performed experimental research on CO 2 crystallization as a multifaceted approach for treating exhaust gases and waste materials such as FA and BA simultaneously. Throughout this research, we implemented a simple process to ensure scalability. In the context of carbon capture, utilization, and storage (CCUS) technology, we conducted experimental research on mineralizing CO 2 targeting FA and BA by applying ambient temperature, atmospheric pressure, and simulated exhaust gas. The empirical findings demonstrated that 12.28 kg CO 2 /ton and 58.14 kg CO 2 /ton of CO 2 were immobilized for BA and FA, respectively. The economic evaluation was measured based on the experimental results obtained from the techno-economic analysis (TEA). The B/C ratio stands at 1.07, with the cost of composite carbonate estimated at USD 159.6 per ton. With an internal rate of return (IRR) of 7.78 % and a net present value (NPV) of USD 7294.59, the economic viability demonstrates considerable promise. Ultimately, this study aims to mitigate the impact of coal-fired power plants on climate change and enhance environmental sustainability through CO 2 removal and waste recycling .
引用
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页数:9
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