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Facile ultrasound-assisted synthesis of g-C3N4@Bi20TiO32/Bi2O2CO3 heterojunction with high photocatalytic performance for resistant-biodegradable dye
被引:2
|作者:
Yan, Yi
[1
]
Li, Danqin
[1
]
Guo, Shenjia
[1
]
Wang, Peijie
[1
]
Ji, Yanyan
[2
]
Zhang, Wu
[1
]
机构:
[1] Tianjin Univ Sci & Technol, Coll Marine & Environm Sci, Tianjin Marine Environm Protect & Restorat Technol, Tianjin Key Lab Marine Resources & Chem, Tianjin 300457, Peoples R China
[2] Tiangong Univ, Sch Chem Engn & Technol, State Key Lab Separat Membranes & Membrane Proc, Tianjin 300387, Peoples R China
基金:
中国国家自然科学基金;
关键词:
Bi20TiO32;
Ternary heterostructure;
Visible photocatalysis;
g-C3N4;
Bi2O2CO3;
CARBON;
DEGRADATION;
FABRICATION;
COMPOSITES;
NANOSHEETS;
D O I:
10.1016/j.jwpe.2024.106162
中图分类号:
X [环境科学、安全科学];
学科分类号:
08 ;
0830 ;
摘要:
In this study, g-C3N4/Bi20TiO32/Bi2O2CO3 photocatalyst structured as a heterojunction was fabricated by an ultrasound-assisted methodology. It evaluated the activity in photocatalytic processes of g-C3N4/Bi20TiO32/Bi2O2CO3 composite material through simulated visible light-induced Rhodamine B photodegradation, demonstrating photodegradation efficiencies 5.6 and 13.84 times exceeding that of pure g-C3N4 and Bi20TiO32/Bi2O2CO3 in turn. Due to the formation of a ternary heterojunction, the g-C3N4/Bi20TiO32/Bi2O2CO3 composite material has a stronger visible light absorption capability compared to pure g-C3N4 and Bi20TiO32/Bi2O2CO3. The photocurrent density is also significantly increased (0.156 mu A/cm(2)). The catalyst's efficiency remained a high degradation ratio (over 95 %) after five cycles, showing the composite's sustainable stability. In summary, based on its excellent performance, the ternary composite photocatalyst g-C3N4/Bi20TiO32/Bi2O2CO3 exhibits great potential for photodegradation of non-biodegradable dye.
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页数:10
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