Facile ultrasound-assisted synthesis of g-C3N4@Bi20TiO32/Bi2O2CO3 heterojunction with high photocatalytic performance for resistant-biodegradable dye

被引:2
|
作者
Yan, Yi [1 ]
Li, Danqin [1 ]
Guo, Shenjia [1 ]
Wang, Peijie [1 ]
Ji, Yanyan [2 ]
Zhang, Wu [1 ]
机构
[1] Tianjin Univ Sci & Technol, Coll Marine & Environm Sci, Tianjin Marine Environm Protect & Restorat Technol, Tianjin Key Lab Marine Resources & Chem, Tianjin 300457, Peoples R China
[2] Tiangong Univ, Sch Chem Engn & Technol, State Key Lab Separat Membranes & Membrane Proc, Tianjin 300387, Peoples R China
基金
中国国家自然科学基金;
关键词
Bi20TiO32; Ternary heterostructure; Visible photocatalysis; g-C3N4; Bi2O2CO3; CARBON; DEGRADATION; FABRICATION; COMPOSITES; NANOSHEETS;
D O I
10.1016/j.jwpe.2024.106162
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
In this study, g-C3N4/Bi20TiO32/Bi2O2CO3 photocatalyst structured as a heterojunction was fabricated by an ultrasound-assisted methodology. It evaluated the activity in photocatalytic processes of g-C3N4/Bi20TiO32/Bi2O2CO3 composite material through simulated visible light-induced Rhodamine B photodegradation, demonstrating photodegradation efficiencies 5.6 and 13.84 times exceeding that of pure g-C3N4 and Bi20TiO32/Bi2O2CO3 in turn. Due to the formation of a ternary heterojunction, the g-C3N4/Bi20TiO32/Bi2O2CO3 composite material has a stronger visible light absorption capability compared to pure g-C3N4 and Bi20TiO32/Bi2O2CO3. The photocurrent density is also significantly increased (0.156 mu A/cm(2)). The catalyst's efficiency remained a high degradation ratio (over 95 %) after five cycles, showing the composite's sustainable stability. In summary, based on its excellent performance, the ternary composite photocatalyst g-C3N4/Bi20TiO32/Bi2O2CO3 exhibits great potential for photodegradation of non-biodegradable dye.
引用
收藏
页数:10
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