Advanced MXene-based materials for efficient extraction of uranium from seawater and wastewater

被引:4
|
作者
Zhu, Jiahui [1 ,2 ,4 ]
Wang, Jing [1 ,2 ,4 ]
Liu, Qi [1 ,2 ,3 ,4 ]
Yu, Jing [1 ,2 ,4 ]
Liu, Jingyuan [1 ,2 ,4 ]
Chen, Rongrong [1 ,2 ,4 ]
Song, Dalei [1 ,2 ,4 ]
Li, Rumin [1 ,2 ,4 ]
Wang, Jun [1 ,2 ]
机构
[1] Harbin Engn Univ, Key Lab Superlight Mat & Surface Technol, Minist Educ, Harbin 150001, Peoples R China
[2] Harbin Engn Univ, Coll Mat Sci & Chem Engn, Harbin 150001, Peoples R China
[3] Hainan Harbin Inst Technol Innovat Res Inst Co Ltd, Hainan 572427, Peoples R China
[4] Minist Ind & Informat Technol, Key Lab Marine Special Mat, Harbin, Peoples R China
基金
中国国家自然科学基金; 中国博士后科学基金;
关键词
MXenes; 2D layered structure; Adsorbents; Uranium extraction; ADSORPTION; REMOVAL; CHEMISTRY; BEHAVIOR; SILICA;
D O I
10.1016/j.scitotenv.2024.173755
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
In order to realize the low -carbon development policy, the large-scale development and utilization of nuclear energy is very essential. Uranium is the key resource for nuclear industry. The extracting and recycling uranium from seawater and nuclear wastewater is necessary for secure uranium reserves, ensure energy security, control pollution and protect the environment. The novel nanomaterial MXene possesses the layered structure, high specific surface area, and modifiable surface terminal groups, which allowed it to enrich uranium. In addition, good photovoltaic and photothermal properties improves the ability to adsorb uranium. The excellent radiation resistance of the MAX phase strongly indicates the potential use of MXene as an effective uranium adsorbent. However, there are relatively few reviews on its application in uranium extraction and recovery. This review focuses on the recent advances in the use of MXene-based materials as highly efficient adsorbents for the recovery of uranium from seawater and nuclear wastewater. First, the structural, synthetic and characterization aspects of MXene materials are introduced. Subsequently, the adsorptive properties of MXene-based materials are evaluated in terms of uranium extraction recovery capability, selectivity, and reproducibility. Furthermore, the interaction mechanisms between uranium and MXene absorbers are discussed. Finally, the challenges for MXene materials in uranium adsorption applications are proposed for better design of new types of MXene-based adsorbents.
引用
收藏
页数:19
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