The Design of a Parameterization Scheme for 137Cs Based on the WRF-Chem Model and Its Application in Simulating the Fukushima Nuclear Accident

Based on the Weather Research and Forecasting Model Coupled with Chemistry (WRF-Chem) atmospheric chemistry model, a parameterization scheme for the radioactive isotope caesium (Cs-137), considering processes such as advection, turbulent diffusion, dry deposition, and wet deposition, was constructed, enabling the spatial distribution simulation of the concentration and deposition of Cs-137. The experimental simulation studies were carried out during the high emission period of the Fukushima nuclear accident (from 11 to 17 March 2011). Two sets of comparison experiments, with or without deposition, were designed, the effects of wind field and precipitation on the spatial transport and ground deposition of Cs-137 were analyzed, and the influence of wind field and precipitation on Cs-137 vertical transport was analyzed in detail. The results indicate that the model can accurately simulate the meteorological and Cs-137 variables. On 15 March, Cs-137 dispersed towards the Kanto Plain in Japan under the influence of northeastern winds. In comparison to the experiment without deposition, the concentration of Cs-137 in the Fukushima area decreased by approximately 286 Bq<middle dot>m(-3) in the deposition experiment. Under the influence of updrafts in the non-deposition experiment, a Cs-137 cloud spread upward to a maximum height of 6 km, whereas in the deposition experiment, the highest dispersion of the Cs-137 cloud only reach a height of 4 km. Affected by the wind field, dry deposition is mainly distributed in Fukushima, the Kanto Plain, and their eastern ocean areas, with a maximum dry deposition of 5004.5 kBq<middle dot>m(-2). Wet deposition is mainly influenced by the wind field and precipitation, distributed in the surrounding areas of Fukushima, with a maximum wet deposition of 725.3 kBq<middle dot>m(-2). The single-station test results from the deposition experiment were better than those for the non-deposition experiment: the percentage deviations of the Tokyo, Chiba, Maebashi, and Naraha stations decreased by 61%, 69%, 46%, and 51%, respectively, and the percentage root mean square error decreased by 46%, 25%, 38%, and 48%, respectively.