Recent advances in silicon nanomaterials for lithium-ion batteries: Synthesis approaches, emerging trends, challenges, and opportunities

被引:3
作者
Hossain, M. A. Motalib [1 ]
Tiong, Sieh Kiong [1 ]
Hannan, M. A. [2 ,3 ]
Ker, Pin Jern [2 ]
Fattah, I. M. R. [4 ]
Mahlia, T. M. Indra [4 ]
机构
[1] Univ Tenaga Nas, Inst Sustainable Energy, Kajang 43000, Malaysia
[2] Sunway Univ, Sch Engn & Technol, Bandar Sunway 47500, Malaysia
[3] Korea Univ, Sch Elect Engn, Seoul 136701, South Korea
[4] Univ Technol Sydney, Sch Civil & Environm Engn, Ultimo, NSW 2007, Australia
关键词
Silicon; Lithium -ion batteries; Energy; Nanomaterials; New trends; HIGH-PERFORMANCE ANODE; IMPROVED ELECTROCHEMICAL PERFORMANCE; CONDUCTIVE POLYMER BINDER; CORE-SHELL STRUCTURE; HIGH-CAPACITY ANODES; IN-SITU GROWTH; ARC-DISCHARGE; FLUOROETHYLENE CARBONATE; NEGATIVE-ELECTRODE; AMORPHOUS-SILICON;
D O I
10.1016/j.susmat.2024.e00964
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Lithium-ion batteries (LIBs) are essential for powering a wide range of current devices, including portable electronics and electric vehicles, because they have a high energy density, can be recharged, and are versatile. Silicon (Si)-based materials are being extensively studied as very promising anode compounds for future LIBs due to their moderate operating potential, high theoretical mass-specific capacity, and abundance. Consequently, it received considerable interest from both the academic and industrial sectors. However, electrochemical efficiency is hindered by significant changes in volume, leading to inadequate cyclability and eventual electrode malfunction. Nanostructured Si anodes address these issues by offering a reduced lithium diffusion distance, effective strain relaxation, improved mass transfer, and efficient electrical contact. The research on Si nanomaterials is highly significant due to the increasing need for improved energy density and safety in the rapidly developing field of energy storage. Recently, there have been attempts to mitigate the negative consequences of bulk effects, and nanosizing has emerged as a widely acknowledged and effective method. However, it has also encountered a limitation in its progress. Hence, this review aims to provide an in-depth overview of recent research on advances in Si materials, synthesis techniques, prevailing trends, and challenges, followed by emphasizing opportunities for future scientific study and commercial development of lithium-ion batteries. Overall, this review study holds significant merit as a reference tool for academics, researchers, and industry to explore research gaps and improve Si-based LIBs, which will shed light on solving the global energy crisis.
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页数:43
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