Engineering silica membranes for separation performance, hydrothermal stability, and production scalability

被引：23

作者：

Bui, Vinh ^{[1
]}

Tandel, Ameya Manoj ^{[1
]}

Satti, Varun Reddy ^{[1
]}

Haddad, Elizabeth ^{[1
]}

Lin, Haiqing ^{[1
]}

机构：

[1] SUNY Buffalo, Dept Chem & Biol Engn, Buffalo, NY 14260 USA

来源：

ADVANCED MEMBRANES | 2023年 / 3卷

基金：

美国国家科学基金会;

关键词：

Silica membranes; Carbon capture; Organosilica membranes; Hydrothermal stability; H; 2; /CO; separation; Scalability; CHEMICAL-VAPOR-DEPOSITION; GAS PERMEATION PROPERTIES; BRIDGED ORGANOSILICA MEMBRANES; REVERSE-OSMOSIS PERFORMANCE; ETHYL LACTATE SYNTHESIS; SOL-GEL; MICROPOROUS SILICA; DOPED SILICA; PORE-SIZE; HYDROGEN SEPARATION;

D O I：

10.1016/j.advmem.2023.100064

中图分类号：

TQ [化学工业];

学科分类号：

0817 ;

摘要：

Silica membranes have been successfully practiced for solvent dehydration and emerged as an exciting platform for gas separations (such as H2/CO2) due to their unique porous structures for molecular sieving, tunable chemistries, and excellent thermal and chemical stability. This review aims to provide a comprehensive update on the advancement of silica membranes for gas and liquid separations in the last decade. First, we summarize various techniques to fabricate membranes (particularly those at low temperatures) and describe the effect of processing parameters on the membrane structures. Second, penetrant transport mechanisms and molecular dynamic simulations are presented to elucidate the structure-properties relationship. Third, we highlight state-ofthe-art silica membranes with promising separation properties for gases, vapors, and liquids and various engineering strategies to improve hydrothermal stability, production scalability, and separation performance. Finally, we provide perspectives on the future development of these membranes for practical applications.

引用

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