A 3D bulk metamaterial (MM) containing amorphous multilayered split-ring resonators is proposed, fabricated, and evaluated. Experimentally, the effective refractive index is engineered via the 3D bulk MM, with a contrast of 0.118 across the frequency span from 0.315 to 0.366 THz and the index changing at a slope of 2.314 per THz within this frequency range. Additionally, the 3D bulk MM exhibits optical isotropy with respect to polarization. Moreover, the peak transmission and optical dispersion are tailored by adjusting the density of the split-ring resonators. Compared to reported conventional approaches for constructing bulk MMs, this approach offers advantages in terms of the potential for large-scale manufacturing, the ability to adopt any shape, optical isotropy, and rapid optical dispersion. These features hold promise for dispersive optical devices operating at THz frequencies, such as high-dispersive prisms for high-resolution spectroscopy. Inspired by natural isotropic materials, a bulk metamaterial composed of amorphous multilayered split-ring resonators is proposed to manipulate the refractive index at terahertz frequencies. Experimental results demonstrate a refractive index variation of 2.314 per terahertz around 0.34 THz incidence frequency. This work exhibits optical isotropy, allows flexible shape design, and supports large-scale manufacturing, providing benefits for dispersive terahertz devices. image