Self-healing PEO/MgAlLa LDHs-MXene composite coating loaded with 4-aminophenol for corrosion protection of Mg-Gd-Y-Zn LPSO Mg alloy

被引:9
作者
Wu, Jiahao [1 ]
Wu, Liang [1 ,2 ]
Yao, Wenhui [1 ,2 ]
Zhou, Yan [1 ]
Wu, Mingyi [1 ]
Yuan, Yuan [1 ,2 ]
Xie, Zhihui [3 ]
Atrens, Andrej [4 ]
Wang, Jingfeng [1 ,2 ]
Pan, Fusheng [1 ,2 ]
机构
[1] Chongqing Univ, Coll Mat Sci & Engn, Natl Engn Res Ctr Magnesium Alloys, Chongqing 400044, Peoples R China
[2] Chongqing Univ, State Key Lab Mech Transmiss, Chongqing 400044, Peoples R China
[3] China West Normal Univ, Coll Chem & Chem Engn, Chem Synth & Pollut Control Key Lab Sichuan Prov, Nanchong 637002, Peoples R China
[4] Univ Queensland, Ctr Adv Mat Proc & Mfg, Sch Mech & Min Engn, St Lucia, Qld 4072, Australia
基金
中国国家自然科学基金;
关键词
Magnesium alloy; MXene@4-Aminophenol material; Corrosion resistance; Self-sealing; Composite coating; LAYERED DOUBLE HYDROXIDE; STACKING ORDERED PHASE; MECHANICAL-PROPERTIES; BEHAVIOR; MICROSTRUCTURE; RESISTANCE; FILMS;
D O I
10.1016/j.electacta.2024.144358
中图分类号
O646 [电化学、电解、磁化学];
学科分类号
081704 ;
摘要
This paper provides an effective method to solve the problems that magnesium alloys easily corrode and their coatings are easily damaged. The micro-pores of PEO coating on the Mg alloy were sealed by in-situ growth of MgAlLa LDHs, and then compounded with MXene doped 4-aminophenol corrosion inhibitor to obtain PEO/ MgAlLa LDHs-MXene@4-Aminophenol (P/MgAlLa LDHs-M@A) composite coating. The structure, morphology and composition of the P/MgAlLa LDHs-M@A coating contained the successful combination of MgAlLa LDHs and MXene@4-Aminophenol. The P/MgAlLa LDHs-M@A coating had excellent corrosion resistance and self-healing properties, with an impedance modulus | Z | 0.01 of 8.8 x 10 7 Omega cm 2 . Scratch defects were self-healed within 12 h. In addition, the mechanisms of corrosion resistance and self-healing were explained.
引用
收藏
页数:20
相关论文
共 73 条
  • [21] Investigation of Corrosion Protection Performance of Multiphase PEO (Mg2SiO4, MgO, MgAl2O4) Coatings on Mg Alloy Formed in Aluminate-Silicate- based Mixture Electrolyte
    Daroonparvar, Mohammadreza
    Yajid, Muhamad Azizi Mat
    Gupta, Rajeev Kumar
    Yusof, Noordin Mohd
    Bakhsheshi-Rad, Hamid Reza
    Ghandvar, Hamidreza
    [J]. PROTECTION OF METALS AND PHYSICAL CHEMISTRY OF SURFACES, 2018, 54 (03) : 425 - 441
  • [22] Effect of particles addition to solution of plasma electrolytic oxidation (PEO) on the properties of PEO coatings formed on magnesium and its alloys: A review
    Fattah-alhosseini, Arash
    Chaharmahali, Razieh
    Babaei, Kazem
    [J]. JOURNAL OF MAGNESIUM AND ALLOYS, 2020, 8 (03) : 799 - 818
  • [23] Conductive two-dimensional titanium carbide 'clay' with high volumetric capacitance
    Ghidiu, Michael
    Lukatskaya, Maria R.
    Zhao, Meng-Qiang
    Gogotsi, Yury
    Barsoum, Michel W.
    [J]. NATURE, 2014, 516 (7529) : 78 - U171
  • [24] Corrosion resistance of AZ31B magnesium alloy with a conversion coating produced from a choline chloride-Urea based deep eutectic solvent
    Gu, C. D.
    Yan, W.
    Zhang, J. L.
    Tu, J. P.
    [J]. CORROSION SCIENCE, 2016, 106 : 108 - 116
  • [25] Layered double hydroxide films: synthesis, properties and applications
    Guo, Xiaoxiao
    Zhang, Fazhi
    Evans, David G.
    Duan, Xue
    [J]. CHEMICAL COMMUNICATIONS, 2010, 46 (29) : 5197 - 5210
  • [26] Effect of phytic acid on the corrosion inhibition of composite film coated on Mg-Gd-Y alloy
    Guo, Xinghua
    Du, Keqin
    Guo, Quanzhong
    Wang, Yong
    Wang, Rong
    Wang, Fuhui
    [J]. CORROSION SCIENCE, 2013, 76 : 129 - 141
  • [27] Effect of Gd and Y contents on the microstructural evolution of long period stacking ordered phase and the corresponding mechanical properties in Mg-Gd-Y-Zn-Mn alloys
    Huang, Song
    Wang, Jingfeng
    Hou, Fan
    Huang, Xiuhong
    Pan, Fusheng
    [J]. MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING, 2014, 612 : 363 - 370
  • [28] Ultrasensitive and selective 4-aminophenol chemical sensor development based on nickel oxide nanoparticles decorated carbon nanotube nanocomposites for green environment
    Hussain, Mohammad Musarraf
    Rahman, Mohammed M.
    Asiri, Abdullah M.
    [J]. JOURNAL OF ENVIRONMENTAL SCIENCES, 2017, 53 : 27 - 38
  • [29] A new Ce-doped MgAl-LDH@Au nanocatalyst for highly efficient reductive degradation of organic contaminants
    Iqbal, Kanwal
    Iqbal, Anam
    Kirillov, Alexander M.
    Wang, Bingkai
    Liu, Weisheng
    Tang, Yu
    [J]. JOURNAL OF MATERIALS CHEMISTRY A, 2017, 5 (14) : 6716 - 6724
  • [30] Effect of starch on the corrosion behavior of Al-Mg-Si alloy processed by micro arc oxidation from an ecofriendly electrolyte system
    Kaseem, Mosab
    Ko, Young Gun
    [J]. BIOELECTROCHEMISTRY, 2019, 128 : 133 - 139