Health Risk Assessment of Heavy Metals in Agricultural Soils Around the Gangue Heap of Coal Mine Based on Monte Carlo Simulation

被引:2
|
作者
Ma J. [1 ,2 ]
She Z.-L. [3 ]
Wang S.-L. [1 ,2 ]
Deng L. [1 ,2 ]
Liu P. [1 ,2 ]
Sun J. [1 ,2 ]
机构
[1] Chongqing Ecological and Environmental Monitoring Center, Chongqing
[2] Rural Ecology and Soil Monitoring Technology Research Center, Chongqing
[3] Chongqing University of Arts and Sciences, Chongqing
来源
Huanjing Kexue/Environmental Science | 2023年 / 44卷 / 10期
关键词
gangue heap of coal mine; health risk assessment; heavy metals; Monte Carlo; soil;
D O I
10.13227/j.hjkx.202211064
中图分类号
学科分类号
摘要
To analyze the pollution characteristics of heavy metals in the soil of farmland surrounding the gangue heap of a coal mine in Chongqing, the Nemerow, Muller, and Hakanson indices were used. Meanwhile, to investigate the health risks of heavy metals in soil, a health risk assessment model was employed using Monte Carlo simulation. The results revealed that the average contents of Cd, Hg, As, Pb, Cr, Cu, Ni, and Zn were higher than their soil background values, and the Muller index (Igeo ) from high to low was as follows: Cd > Hg > Cu > As > Ni > Zn > Cr > Pb. The Nemerow index (PN ) demonstrated that the results of the assessment indicated mainly light pollution (1 < PN 臆2). The single factor index (Pi ) from high to low was as follows: Cd > Cu > Ni > Cr > Zn > As > Pb > Hg. The Hakanson index (RI) demonstrated that the results of the assessment indicated mainly moderate ecological risk (150臆RI <300). The single ecological risk index (Eir ) from high to low was as follows: Cd > Hg > As > Cu > Ni > Pb > Cr > Zn. The health risk assessment of heavy metals revealed that the non-carcinogenic health risks of children and adults could be ignored, but carcinogenic health risks existed, with an average total carcinogenic risk index (TCR) of 1. 04E -5 and 3. 94E -6, respectively. The major carcinogenic factors were As and Cd. Sensitivity analysis of non-carcinogenic health risks revealed that the ingestion rate of soil (Ringest ) was the most sensitive, followed by the contents of As. Meanwhile, sensitivity analysis of carcinogenic health risks indicated that the content of As was the most sensitive, followed by the ingestion rate of soil (Ringest ). In general, the health risks of children, including non-carcinogenic and carcinogenic risks, were higher than those of adults. © 2023 Science Press. All rights reserved.
引用
收藏
页码:5666 / 5678
页数:12
相关论文
共 58 条
  • [1] Kang H P, Wang G F, Wang S M, Et al., High-quality development of China's coal industry, Strategic Study of CAE, 23, 5, pp. 130-138, (2021)
  • [2] Liu F, Cao W J, Zhang J M, Et al., Current technological innovation and development direction of the 14<sup>th</sup> five-year plan period in China coal industry, Journal of China Coal Society, 46, 1, pp. 1-15, (2021)
  • [3] Li J Y, Wang J M., Comprehensive utilization and environmental risks of coal gangue: a review, Journal of Cleaner Production, 239, (2019)
  • [4] Wang J, Wei Z Y, Wang Q B., Evaluating the eco-environment benefit of land reclamation in the dump of an opencast coal mine [J], Chemistry and Ecology, 33, 7, pp. 607-624, (2017)
  • [5] Ge H, Feng Y, Li Y, Et al., Heavy metal pollution diagnosis and ecological risk assessment of the surrounding soils of coal waste pile at Naluo coal mine, Liupanshui, Guizhou[J], International Journal of Mining, Reclamation and Environment, 30, 4, pp. 312-318, (2016)
  • [6] Stracher G B, Taylor T P., Coal fires burning out of control around the world: thermodynamic recipe for environmental catastrophe[J], International Journal of Coal Geology, 59, 1-2, pp. 7-17, (2004)
  • [7] Zhou X H, Shu Y, Zhou L L, Et al., Study on effects of pH value on alkalinity and heavy metal release of alkaline coal gangue, Journal of Safety and Environment, 22, 5, pp. 2752-2758, (2022)
  • [8] Rodriguez R, Diaz M B, Vigil H, Et al., Development of a user-friendly method to assess the present condition of old abandoned mining waste dumps in Asturias (Spain) [J], International Journal of Mining, Reclamation and Environment, 25, 1, pp. 6-31, (2011)
  • [9] Ma J, Liu P, Liu J Z, Et al., Pollution evaluation and quantitative traceability analysis of heavy metals in farmland soils around the gangue heap of a coal mine in Chongqing, Environmental Science, 43, 12, pp. 5698-5709, (2022)
  • [10] Cao S Z, Duan X L, Zhao X G, Et al., Health risks from the exposure of children to As, Se, Pb and other heavy metals near the largest coking plant in China, Science of the Total Environment, 472, pp. 1001-1009, (2014)