Prediction of atmospheric pollutants in urban environment based on coupled deep learning model and sensitivity analysis

被引:12
作者
Wang S. [1 ,2 ]
Ren Y. [2 ]
Xia B. [2 ]
Liu K. [1 ]
Li H. [1 ]
机构
[1] School of Environment, Nanjing Normal University, Nanjing
[2] School of Mathematics and Computer Science, Yan'an University, Yan'an
关键词
Atmospheric pollutants; Attention mechanism; Convolutional neural network; Long short-term memory network; Sensitivity analysis;
D O I
10.1016/j.chemosphere.2023.138830
中图分类号
学科分类号
摘要
Accurate and efficient predictions of pollutants in the atmosphere provide a reliable basis for the scientific management of atmospheric pollution. This study develops a model that combines an attention mechanism, convolutional neural network (CNN), and long short-term memory (LSTM) unit to predict the O3 and PM2.5 levels in the atmosphere, as well as an air quality index (AQI). The prediction results given by the proposed model are compared with those from CNN-LSTM and LSTM models as well as random forest and support vector regression models. The proposed model achieves a correlation coefficient between the predicted and observed values of more than 0.90, outperforming the other four models. The model errors are also consistently lower when using the proposed approach. Sobol-based sensitivity analysis is applied to identify the variables that make the greatest contribution to the model prediction results. Taking the COVID-19 outbreak as the time boundary, we find some homology in the interactions among the pollutants and meteorological factors in the atmosphere during different periods. Solar irradiance is the most important factor for O3, CO is the most important factor for PM2.5, and particulate matter has the most significant effect on AQI. The key influencing factors are the same over the whole phase and before the COVID-19 outbreak, indicating that the impact of COVID-19 restrictions on AQI gradually stabilized. Removing variables that contribute the least to the prediction results without affecting the model prediction performance improves the modeling efficiency and reduces the computational costs. © 2023 Elsevier Ltd
引用
收藏
相关论文
共 68 条
[1]  
Altuwayjiri A., Soleimanian E., Moroni S., Palomba P., Borgini A., De Marco C., Ruprecht A.A., Sioutas C., The impact of stay-home policies during Coronavirus-19 pandemic on the chemical and toxicological characteristics of ambient PM2. 5 in the metropolitan area of Milan, Italy, Sci. Total Environ., 758, (2021)
[2]  
Analitis A., Barratt B., Green D., Beddows A., Samoli E., Schwartz J., Katsouyanni K., Prediction of PM2. 5 concentrations at the locations of monitoring sites measuring PM10 and NOx, using generalized additive models and machine learning methods: a case study in London, Atmos. Environ., 240, (2020)
[3]  
Azodi C.B., Tang J., Shiu S.-H., Opening the black box: interpretable machine learning for geneticists, Trends Genet., 36, pp. 442-455, (2020)
[4]  
Barbhuiya A.A., Karsh R.K., Jain R., CNN based feature extraction and classification for sign language, Multimed. Tool. Appl., 80, pp. 3051-3069, (2021)
[5]  
Benish S.E., He H., Ren X., Roberts S.J., Salawitch R.J., Li Z., Wang F., Wang Y., Zhang F., Shao M., Measurement report: aircraft observations of ozone, nitrogen oxides, and volatile organic compounds over Hebei Province, China, Atmos. Chem. Phys., 20, pp. 14523-14545, (2020)
[6]  
Bowe B., Xie Y., Li T., Yan Y., Xian H., Al-Aly Z., The 2016 global and national burden of diabetes mellitus attributable to PM2· 5 air pollution, Lancet Planet. Health, 2, pp. e301-e312, (2018)
[7]  
Campos V.P., Cruz L.P., Godoi R.H., Godoi A.F.L., Tavares T.M., Development and validation of passive samplers for atmospheric monitoring of SO2, NO2, O3 and H2S in tropical areas, Microchem. J., 96, pp. 132-138, (2010)
[8]  
Chen Y., Schleicher N., Cen K., Liu X., Yu Y., Zibat V., Dietze V., Fricker M., Kaminski U., Chen Y., Evaluation of impact factors on PM2. 5 based on long-term chemical components analyses in the megacity Beijing, China, Chemosphere, 155, pp. 234-242, (2016)
[9]  
Chu J., Dong Y., Han X., Xie J., Xu X., Xie G., Short-term prediction of urban PM2. 5 based on a hybrid modified variational mode decomposition and support vector regression model, Environ. Sci. Pollut. Control Ser., 28, pp. 56-72, (2021)
[10]  
Chuang M.-T., Zhang Y., Kang D., Application of WRF/Chem-MADRID for real-time air quality forecasting over the Southeastern United States, Atmos. Environ., 45, pp. 6241-6250, (2011)