Preparation, modification and the application in catalytic hydrogenation of graphitic carbon nitride

被引：0

作者：

Li S. ^{[1
]}

Yao N. ^{[1
]}

机构：

[1] State Key Laboratory Breeding Base of Green Chemistry Synthesis Technology, Industrial Catalysis Institute, Zhejiang University of Technology, Hangzhou

来源：

Gao Xiao Hua Xue Gong Cheng Xue Bao/Journal of Chemical Engineering of Chinese Universities | 2020年 / 34卷 / 05期

关键词：

Catalytic hydrogenation; Graphitic carbon nitride; Modification; Preparation method; Supported metal catalyst;

D O I：

10.3969/j.issn.1003-9015.2020.05.001

中图分类号：

学科分类号：

摘要：

Graphitic carbon nitride (g-C3N4) is a metal-free polymeric semiconductor material and has unique physicochemical properties and electronic structure, and has great application potential in heterogeneous catalytic hydrogenation in recent years. This paper introduced main preparation methods of g-C3N4 (e.g. hard template method, soft template method and template-free method) and the modification methods (e.g. doping with non-metal atoms/metal atoms and compounding with other materials). It also summarized the recent progresses in the application of g-C3N4 supported metal catalyst in the catalytic hydrogenation of fine chemicals, C1 molecules, alkenes and alkynes, and discussed the development trend and key problems in the related field. © 2020, Editorial Board of Journal of Chemical Engineering of Chinese Universities". All right reserved."

引用

页码：1091 / 1101

页数：10

共 75 条

[1]

CHEN P, TANG C L, ZHAO M H, Et al., Kinetic study on hydrogenation of 2,4-dinitrotoluene to 2,4-tolylenediamine catalyzed by Ni/HY catalysts, Journal of Chemical Engineering of Chinese Universities, 32, 5, pp. 1119-1126, (2018)

[2]

LI K, ZHOU Y, ZHANG Q F, Et al., Preparation of doped carbon materials and their application in catalytic hydrogenation loaded with noble metals, Journal of Chemical Engineering of Chinese Universities, 33, 3, pp. 516-523, (2019)

[3]

GONG Y T, LI M M, LI H R, Et al., Graphitic carbon nitride polymers: promising catalysts or catalyst supports for heterogeneous oxidation and hydrogenation, Green Chemistry, 17, 2, pp. 715-736, (2015)

[4]

WANG Y, WANG X C, ANTONIETTI M., Polymeric graphitic carbon nitride as a heterogeneous organocatalyst: From photochemistry to multipurpose catalysis to sustainable chemistry, Angewandte Chemie, 51, 1, pp. 68-89, (2012)

[5]

DAI X Q, ZHU Y B, XU X L, Et al., Photocatalysis with g-C3N4 applied to organic synthesis, Chinese Journal of Organic Chemistry, 37, 3, pp. 577-585, (2017)

[6]

TONG Z W, YANG D, XIAO T X, Et al., Biomimetic fabrication of g-C3N4/TiO2 nanosheets with enhanced photocatalytic activity toward organic pollutant degradation, Chemical Engineering Journal, 260, pp. 117-125, (2015)

[7]

WANG X C, MAEDA K, THOMAS A, Et al., A metal-free polymeric photocatalyst for hydrogen production from water under visible light, Nature Materials, 8, 1, pp. 76-80, (2009)

[8]

GOETTMANN F, FISCHER A, ANTONIETTIi M, Et al., Chemical synthesis of mesoporous carbon nitrides using hard templates and their use as a metal-free catalyst for Friedel-Crafts reaction of benzene, Angewandte Chemie, 45, 27, pp. 4467-4471, (2006)

[9]

ZHENG Y, JIAO Y, ZHU Y H, Et al., Molecule-level g-C3N4 coordinated transition metals as a new class of electrocatalysts for oxygen electrode reactions, Journal of the American Chemical Society, 139, 9, pp. 3336-3339, (2017)

[10]

TAHIR B, TAHIR M, AMIN N A S., Photo-induced CO2 reduction by CH4/H2O to fuels over Cu-modified g-C3N4 nanorods under simulated solar energy, Applied Surface Science, 419, pp. 875-885, (2017)

← 1 2 3 4 5 6 7 8 →