Polydopamine Assisted Co-Assembly for Fabrication of Zwitterionic Polymer Nanocoating with Efficient Aqueous Lubrication

被引:0
|
作者
Wei Q. [1 ]
Yue Q. [1 ]
Li L. [1 ]
Fu T. [1 ]
Ma S. [2 ]
Zhou F. [2 ]
机构
[1] Key Laboratory of Polymer Materials of Gansu Province, College of Chemistry and Chemical Engineering, Northwest Normal University, Lanzhou, 730070, Gansu
[2] State Key Laboratory of Solid Lubrication, Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences, Lanzhou, 730000, Gansu
来源
Mocaxue Xuebao/Tribology | 2019年 / 39卷 / 04期
基金
中国国家自然科学基金;
关键词
Aqueous lubrication; Low friction coating; Polydopamine; Surface modification; Zwitterionic polymer;
D O I
10.16078/j.tribology.2019069
中图分类号
学科分类号
摘要
Low friction and hydrophilic surfaces have critical applications in biomedical devices and implants. This work reports a facile and universal method to prepare hydrophilic, low friction and antifouling coating by dopamine assisted codeposition of chitosan graft zwitterionic copolymer. The effects of polymer concentration on the thickness, hydrophilicity and lubricity of co-deposited coatings were investigated. The results show that the coating thickness decreases slightly with the increase of polymer concentration. The codeposited coating shows superior lubrication performance (friction coefficient μ is 0.015) and antifouling in pure water as well as biological fluids. Furthermore, the versatility of this strategy allows fabrication of lubricious polymer coatings on diverse materials surfaces. This multifunctional coating may find important applications in biomedical devices and implants. © 2019, Science Press. All right reserved.
引用
收藏
页码:387 / 395
页数:8
相关论文
共 29 条
  • [1] Lamprou D., Scoutaris N., Ross S., Et al., Polymeric coatings and their fabrication for medical devices., Encyclopedia of Biomedical Engineering, pp. 177-187, (2019)
  • [2] Albers P.T.M., Govers S.P.W., Laven J., Et al., Design of dual hydrophobic-hydrophilic polymer networks for highly lubricious polyether-urethane coatings, European Polymer Journal, 111, pp. 82-94, (2019)
  • [3] Van Bochove B., Rongen J.J., Hannink G., Et al., Grafting a lubricious coating onto photo-crosslinked poly (trimethylene carbonate), Polymers for Advanced Technologies, 26, 12, pp. 1428-1432, (2015)
  • [4] Mccutchen C.W., The frictional properties of animal joints, Wear, 5, 1, pp. 1-17, (1962)
  • [5] Neville A., Morina A., Liskiewicz T., Et al., Synovial joint lubrication-does nature teach more effective engineering lubrication strategies, Proceedings of the Institution of Mechanical Engineers, Part C: Journal of Mechanical Engineering Science, 221, 10, pp. 1223-1230, (2007)
  • [6] Jahn S., Seror J., Klein J., Lubrication of articular cartilage, Annual Review of Biomedical Engineering, 18, pp. 235-258, (2016)
  • [7] Liu G., Guo W., Liu Z., Et al., Research progress on polymer-based biomimetic lubricants, Tribology, 35, 1, pp. 108-120, (2015)
  • [8] Morgese G., Benetti E.M., Zenobi Wong M., Molecularly engineered biolubricants for articular cartilage, Advanced Healthcare Materials, 7, 16, (2018)
  • [9] Singh A., Corvelli M., Unterman S.A., Et al., Enhanced lubrication on tissue and biomaterial surfaces through peptide-mediated binding of hyaluronic acid, Nature Materials, 13, 10, pp. 988-995, (2014)
  • [10] Sterner O., Karageorgaki C., Zurcher M., Et al., Reducing friction in the eye: a comparative study of lubrication by surface-anchored synthetic and natural ocular mucin analogues, ACS Applied Materials & Interfaces, 9, 23, pp. 20150-20160, (2017)