Measurement of effective 98Mo(n,γ)99 Mo reaction cross-section in the epi-cadmium neutron flux produced by 10 MeV electron LINAC with Ta-BeO assembly

被引:1
作者
Deo, Kapil [1 ]
Kumar, Rajeev [1 ,2 ]
Mallick, Amod K. [1 ]
Samanta, Sudipta [1 ]
Bhandari, Deep [1 ]
Sarkar, Anindita [1 ]
Umasankari, K. [1 ,2 ]
Chaudhary, Nishant [2 ,3 ]
Pant, Amar D. [4 ]
Verma, Amit [4 ]
Anilkumar, P. [4 ]
机构
[1] Bhabha Atom Res Ctr, Reactor Phys Design Div, Mumbai 400085, India
[2] Bhabha Atom Res Ctr, Homi Bhabha Natl Inst, Mumbai 400085, India
[3] Bhabha Atom Res Ctr, Accelerator & Pulse Power Div, Mumbai 400085, India
[4] Bhabha Atom Res Ctr, Environm Monitoring & Assessment Div, Mumbai 400085, India
关键词
Mo-98(n; gamma)Mo-99; reaction; Mo-99/Tc-99m Medical radioisotopes; Electron accelerator; Epi-cadmium neutrons; Ta-BeO assembly; NUCLEAR-REACTOR; MO-99; MO-100(GAMMA; ENERGY; NAT;
D O I
10.1007/s10967-024-09521-7
中图分类号
O65 [分析化学];
学科分类号
070302 ; 081704 ;
摘要
An experiment was carried out to study the feasibility of Mo-99 production using an electron accelerator based epi-cadmium neutron source. The neutrons were produced by the interaction of bremsstrahlung end-point energy of 10 MeV with BeO blocks and the neutrons thus produced were moderated using High Density Polyethylene blocks. Effective cross-section of Mo-98(n,gamma)Mo-99 reaction was measured using foil activation method. An enhancement in the effective cross-section due to resonances in the epi-cadmium region was observed. The photons and neutron production/transport in the experimental set-up were simulated using the FLUKA Monte Carlo code. The simulations were found to be in good agreement with the experimental findings.
引用
收藏
页码:3793 / 3806
页数:14
相关论文
共 25 条
[1]  
[Anonymous], 2021, E26116 ASTM INT
[2]  
[Anonymous], 2005, CERN-2005-10, INFN/TC_05/11, SLAC-R-773
[3]  
[Anonymous], about us
[4]   Measurement of formation cross-section of 99Mo from the 98Mo(n,γ) and 100Mo,2n) reactions [J].
Badwar, Sylvia ;
Ghosh, Reetuparna ;
Lawriniang, Bioletty M. ;
Vansola, Vibha ;
Sheela, Y. S. ;
Naik, Haladhara ;
Naik, Yeshwant ;
Suryanarayana, Saraswatula V. ;
Jyrwa, Betylda ;
Ganesan, Srinivasan .
APPLIED RADIATION AND ISOTOPES, 2017, 129 :117-123
[5]   Overview of the FLUKA code [J].
Battistoni, Giuseppe ;
Boehlen, Till ;
Cerutti, Francesco ;
Chin, Pik Wai ;
Esposito, Luigi Salvatore ;
Fasso, Alberto ;
Ferrari, Alfredo ;
Lechner, Anton ;
Empl, Anton ;
Mairani, Andrea ;
Mereghetti, Alessio ;
Ortega, Pablo Garcia ;
Ranft, Johannes ;
Roesler, Stefan ;
Sala, Paola R. ;
Vlachoudis, Vasilis ;
Smirnov, George .
ANNALS OF NUCLEAR ENERGY, 2015, 82 :10-18
[6]   Determination of spectrum shaping factor in nuclear reactor AHWR-CF by Monte Carlo method for material characterization using neutrons [J].
Bhandari, Deep ;
Mallick, Amod Kishore ;
Samanta, Sudipta ;
Sarkar, Anindita ;
Kumar, Rajeev ;
Kannan, Umasankari .
MATERIALS TODAY-PROCEEDINGS, 2021, 38 :3041-3045
[7]   The FLUKA Code: Developments and Challenges for High Energy and Medical Applications [J].
Boehlen, T. T. ;
Cerutti, F. ;
Chin, M. P. W. ;
Fosso, A. ;
Ferrari, A. ;
Ortega, P. G. ;
Mairani, A. ;
Sala, P. R. ;
Smirnov, G. ;
Vlachoudisl, V. .
NUCLEAR DATA SHEETS, 2014, 120 :211-214
[8]   99mTc by 99Mo produced at the ENEA-FNG facility of 14 MeV neutrons [J].
Capogni, M. ;
Pietropaolo, A. ;
Quintieri, L. ;
Fazio, A. ;
De Felice, P. ;
PiIlon, M. ;
Pizzuto, A. .
APPLIED RADIATION AND ISOTOPES, 2018, 134 :105-107
[9]   Photo-neutron cross-section of 100Mo [J].
Crasta, Rita ;
Naik, H. ;
Suryanarayana, S. V. ;
Prajapati, P. M. ;
Jagadisan, K. C. ;
Thakare, S. V. ;
Ganesh, S. ;
Nimje, V. T. ;
Mittal, K. C. ;
Goswami, A. .
JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY, 2011, 290 (02) :367-373
[10]   Estimation of photoneutron yield from beryllium target irradiated by variable energy microtron-based bremsstrahlung radiation [J].
Eshwarappa, KM ;
Ganesh ;
Siddappa, K ;
Kashyap, Y ;
Sinha, A ;
Sarkar, PS ;
Godwal, BK .
NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT, 2005, 540 (2-3) :412-418