Biogas;
Biomethanol;
Carbon capture;
Energy conversion;
Energy storage;
CATALYTIC METHANATION;
SWING ADSORPTION;
CO2;
EQUILIBRIUM;
REMOVAL;
REACTOR;
13X;
D O I:
10.1002/cite.202300200
中图分类号:
TQ [化学工业];
学科分类号:
0817 ;
摘要:
Coupling of biogas upgrading and power-to-X is challenging due to the intermittent cheap energy availability. A system was designed that overcomes the technical challenges in this coupling. This is possible by alternating biogas upgrading and methanol synthesis in a reactor operating both as sorption-enhanced synthesis reactor and as upgrading unit by pressure swing adsorption. It was observed that this concept is feasible in both fixed- and fluidized-bed reactors, and the potential for economic performance improvement was quantified in approximately 20 % increase of the internal rate of return. A flexible reactor that operates both the CO2 conversion to methanol and the CO2 separation is conceptualized. The flexible process shows high economic potential to advance the penetration of power-to-X routes. image
机构:
Paul Scherrer Inst, Energy & Environm Res Div, CH-5232 Villigen, SwitzerlandPaul Scherrer Inst, Energy & Environm Res Div, CH-5232 Villigen, Switzerland
Calbry-Muzyka, Adelaide S.
Gantenbein, Andreas
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机构:
Paul Scherrer Inst, Energy & Environm Res Div, CH-5232 Villigen, SwitzerlandPaul Scherrer Inst, Energy & Environm Res Div, CH-5232 Villigen, Switzerland
Gantenbein, Andreas
Schneebeli, Jorg
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机构:
Paul Scherrer Inst, Energy & Environm Res Div, CH-5232 Villigen, SwitzerlandPaul Scherrer Inst, Energy & Environm Res Div, CH-5232 Villigen, Switzerland
Schneebeli, Jorg
Frei, Alwin
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机构:
Paul Scherrer Inst, Energy & Environm Res Div, CH-5232 Villigen, SwitzerlandPaul Scherrer Inst, Energy & Environm Res Div, CH-5232 Villigen, Switzerland
Frei, Alwin
Knorpp, Amy J.
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h-index: 0
机构:
Swiss Fed Inst Technol, Vladimir Prelog Weg 1, CH-8093 Zurich, SwitzerlandPaul Scherrer Inst, Energy & Environm Res Div, CH-5232 Villigen, Switzerland
Knorpp, Amy J.
Schildhauer, Tilman J.
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h-index: 0
机构:
Paul Scherrer Inst, Energy & Environm Res Div, CH-5232 Villigen, SwitzerlandPaul Scherrer Inst, Energy & Environm Res Div, CH-5232 Villigen, Switzerland
Schildhauer, Tilman J.
Biollaz, Serge M. A.
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h-index: 0
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Paul Scherrer Inst, Energy & Environm Res Div, CH-5232 Villigen, SwitzerlandPaul Scherrer Inst, Energy & Environm Res Div, CH-5232 Villigen, Switzerland
机构:
INCAR CSIC, Inst Ciencia & Tecnol Carbono, C Francisco Pintado Fe 26, Oviedo 33011, SpainINCAR CSIC, Inst Ciencia & Tecnol Carbono, C Francisco Pintado Fe 26, Oviedo 33011, Spain
Duran, Ines
Rubiera, Fernando
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INCAR CSIC, Inst Ciencia & Tecnol Carbono, C Francisco Pintado Fe 26, Oviedo 33011, SpainINCAR CSIC, Inst Ciencia & Tecnol Carbono, C Francisco Pintado Fe 26, Oviedo 33011, Spain
Rubiera, Fernando
Pevida, Covadonga
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h-index: 0
机构:
INCAR CSIC, Inst Ciencia & Tecnol Carbono, C Francisco Pintado Fe 26, Oviedo 33011, SpainINCAR CSIC, Inst Ciencia & Tecnol Carbono, C Francisco Pintado Fe 26, Oviedo 33011, Spain
机构:
Paul Scherrer Inst, Energy & Environm Res Div, CH-5232 Villigen, SwitzerlandPaul Scherrer Inst, Energy & Environm Res Div, CH-5232 Villigen, Switzerland
Calbry-Muzyka, Adelaide S.
Gantenbein, Andreas
论文数: 0引用数: 0
h-index: 0
机构:
Paul Scherrer Inst, Energy & Environm Res Div, CH-5232 Villigen, SwitzerlandPaul Scherrer Inst, Energy & Environm Res Div, CH-5232 Villigen, Switzerland
Gantenbein, Andreas
Schneebeli, Jorg
论文数: 0引用数: 0
h-index: 0
机构:
Paul Scherrer Inst, Energy & Environm Res Div, CH-5232 Villigen, SwitzerlandPaul Scherrer Inst, Energy & Environm Res Div, CH-5232 Villigen, Switzerland
Schneebeli, Jorg
Frei, Alwin
论文数: 0引用数: 0
h-index: 0
机构:
Paul Scherrer Inst, Energy & Environm Res Div, CH-5232 Villigen, SwitzerlandPaul Scherrer Inst, Energy & Environm Res Div, CH-5232 Villigen, Switzerland
Frei, Alwin
Knorpp, Amy J.
论文数: 0引用数: 0
h-index: 0
机构:
Swiss Fed Inst Technol, Vladimir Prelog Weg 1, CH-8093 Zurich, SwitzerlandPaul Scherrer Inst, Energy & Environm Res Div, CH-5232 Villigen, Switzerland
Knorpp, Amy J.
Schildhauer, Tilman J.
论文数: 0引用数: 0
h-index: 0
机构:
Paul Scherrer Inst, Energy & Environm Res Div, CH-5232 Villigen, SwitzerlandPaul Scherrer Inst, Energy & Environm Res Div, CH-5232 Villigen, Switzerland
Schildhauer, Tilman J.
Biollaz, Serge M. A.
论文数: 0引用数: 0
h-index: 0
机构:
Paul Scherrer Inst, Energy & Environm Res Div, CH-5232 Villigen, SwitzerlandPaul Scherrer Inst, Energy & Environm Res Div, CH-5232 Villigen, Switzerland
机构:
INCAR CSIC, Inst Ciencia & Tecnol Carbono, C Francisco Pintado Fe 26, Oviedo 33011, SpainINCAR CSIC, Inst Ciencia & Tecnol Carbono, C Francisco Pintado Fe 26, Oviedo 33011, Spain
Duran, Ines
Rubiera, Fernando
论文数: 0引用数: 0
h-index: 0
机构:
INCAR CSIC, Inst Ciencia & Tecnol Carbono, C Francisco Pintado Fe 26, Oviedo 33011, SpainINCAR CSIC, Inst Ciencia & Tecnol Carbono, C Francisco Pintado Fe 26, Oviedo 33011, Spain
Rubiera, Fernando
Pevida, Covadonga
论文数: 0引用数: 0
h-index: 0
机构:
INCAR CSIC, Inst Ciencia & Tecnol Carbono, C Francisco Pintado Fe 26, Oviedo 33011, SpainINCAR CSIC, Inst Ciencia & Tecnol Carbono, C Francisco Pintado Fe 26, Oviedo 33011, Spain