Research on purification, combustion and NOx emission characteristics of pulverized coal preheated by a novel self-sustained purifying burner

被引:6
作者
Su, Kun [1 ,2 ]
Ouyang, Ziqu [1 ,2 ]
Wang, Hongshuai [1 ,2 ]
Zhang, Jinyang [1 ,3 ]
Ding, Hongliang [1 ,2 ]
Wang, Wenyu [1 ,2 ]
机构
[1] Chinese Acad Sci, Inst Engn Thermophys, 11Beisihuanxi Rd, Beijing 100190, Peoples R China
[2] Univ Chinese Acad Sci, Beijing 100049, Peoples R China
[3] Jiangsu Univ, Zhenjiang 212013, Peoples R China
关键词
Purification characteristic; Combustion characteristic; NOx emission; Purifying temperature; NITROGEN; TEMPERATURE; GAS; CO2; SPECTROSCOPY; PYROLYSIS; CHINA;
D O I
10.1016/j.fuel.2024.131436
中图分类号
TE [石油、天然气工业]; TK [能源与动力工程];
学科分类号
0807 ; 0820 ;
摘要
To more quickly achieve the breakthrough of minimum NOx emission, this study focused on purification, combustion and NOx emission characteristics of pulverized coal preheated by a novel self-sustained purifying burner, and deeply explored the effect of purifying temperature (T-p) in a 30 kW purification-combustion system. In the purifying burner, the main combustible gases in the reductive coal gas were CO and H-2, and their concentrations ranked as CO > H-2. Increasing T-p rose their yields. By contrast, the CH4 concentration was always extremely low. This burner effectively improved the particle properties of pulverized coal (including particle size, macrostructure, carbon microcrystalline structure and fuel conversion rate), and was superior over the previous self-preheating burner. Properly increasing T-p optimized the particle properties of reductive coal char except pore diameter, and there might be an optimal T-p. The pore diameter always decreased as T-p increased. Increasing T-p reduced the relative content of N-X in the reductive coal char, and its content was extremely low when T-p was above 1083 degrees C. Moreover, N-Q was the main form of nitrogen functional groups in the reductive coal char at an extremely high T-p. In the subsequent combustion, NO2 and NO were the main forms of nitrogen oxides in the reduction and burnout regions respectively, while N2O was not. In the whole purification-combustion system, the burning efficiency was always about 99.50 %, and its change was extremely small as T-p increased, while the NOx emission decreased first and then increased. Moreover, the adverse effect of higher T-p on the emission was more significant compared to lower T-p.
引用
收藏
页数:14
相关论文
共 65 条
  • [11] Experimental study on the influence of O2/CO2 ratios on NO conversion and emission during combustion and gasification of high-temperature coal char
    Ding, Hongliang
    Ouyang, Ziqu
    Wang, Wenyu
    Zhang, Xiaoyu
    Zhu, Shujun
    [J]. FUEL, 2022, 310
  • [12] The effects of particle size on flameless combustion characteristics and NOx emissions of semi-coke with coal
    Ding, Hongliang
    Ouyang, Ziqu
    Zhang, Xiaoyu
    Zhu, Shujun
    [J]. FUEL, 2021, 297
  • [13] Gaseous emissions from the combustion of a waste mixture containing a high concentration of N2O
    Dong, Changqing
    Yang, Yongping
    Zhang, Junjiao
    Lu, Xuefeng
    [J]. WASTE MANAGEMENT, 2009, 29 (01) : 272 - 276
  • [14] Thermogravimetric analysis of gasification reactivity of coal chars with steam and CO2 at moderate temperatures
    Dongmei Fan
    Zhiping Zhu
    Yongjie Na
    Qinggang Lu
    [J]. Journal of Thermal Analysis and Calorimetry, 2013, 113 (2) : 599 - 607
  • [15] Microstructure and its influence on CH4 adsorption behavior of deep coal
    Feng Yan-Yan
    Jiang Cheng-Fa
    Liu Dai-Jun
    Chu Wei
    [J]. CHINESE PHYSICS B, 2014, 23 (02)
  • [16] Effect of Coal Consumption on the Upgrading of Industrial Structure
    Guo, Xuyang
    Wang, Xin
    Zheng, Dezhi
    [J]. GEOFLUIDS, 2022, 2022
  • [17] Analysis of low NO emission in high temperature air combustion for pulverized coal
    He, R
    Suda, T
    Takafuji, M
    Hirata, T
    Sato, J
    [J]. FUEL, 2004, 83 (09) : 1133 - 1141
  • [18] The Influence of Biomass Gasification Gas on the Reduction of N2O Emissions in a Fluidized Bed
    Hu, X.
    Dong, C.
    Lu, Q.
    Zhang, J.
    Zhang, H.
    Dong, Z.
    Yang, Y.
    [J]. ENERGY SOURCES PART A-RECOVERY UTILIZATION AND ENVIRONMENTAL EFFECTS, 2013, 35 (15) : 1410 - 1417
  • [19] Characteristics of particulate matter generated in pressurized coal combustion for high-efficiency power generation system
    Kurose, R
    Matsuda, H
    Makino, H
    Suzuki, A
    [J]. ADVANCED POWDER TECHNOLOGY, 2003, 14 (06) : 673 - 694
  • [20] CFD predictions of wake-stabilised jet flames in a cross-flow
    Lawal, Mohammed S.
    Fairweather, Michael
    Gogolek, Peter
    Ingham, Derek B.
    Ma, Lin
    Pourkashanian, Mohamed
    Williams, Alan
    [J]. ENERGY, 2013, 53 : 259 - 269