Noncoplanar magnetic order in the breathing kagome lattice compound Pb(OF)Cu3(SeO3)2(NO3)

被引：3

作者：

Gu, Yimeng ^{[1
,2
,3
]}

Kao, Zeyu ^{[1
,2
,3
]}

Hao, Yiqing ^{[4
]}

Zhu, Weiqin ^{[1
,2
,3
]}

Zhang, Qiang ^{[4
]}

Wu, Yan ^{[4
]}

Xu, Changsong ^{[1
,2
,3
]}

Cao, Huibo ^{[4
]}

Zhao, Jun ^{[1
,2
,3
,5
,6
,7
]}

机构：

[1] Fudan Univ, State Key Lab Surface Phys, Shanghai 200433, Peoples R China

[2] Fudan Univ, Dept Phys, Shanghai 200433, Peoples R China

[3] Shanghai Qi Zhi Inst, Shanghai 200230, Peoples R China

[4] Oak Ridge Natl Lab, Neutron Scattering Div, Oak Ridge, TN 37831 USA

[5] Fudan Univ, Inst Nanoelect Devices & Quantum Comp, Shanghai 200433, Peoples R China

[6] Shanghai Res Ctr Quantum Sci, Shanghai 201315, Peoples R China

[7] Collaborat Innovat Ctr Adv Microstruct, Nanjing 210093, Peoples R China

来源：

PHYSICAL REVIEW B | 2024年 / 109卷 / 02期

基金：

中国国家自然科学基金;

关键词：

BILBAO CRYSTALLOGRAPHIC SERVER; GROUND-STATE; JAROSITES; MODEL;

D O I：

10.1103/PhysRevB.109.024402

中图分类号：

T [工业技术];

学科分类号：

08 ;

摘要：

We report a comprehensive study investigating the magnetic ordering properties of the quasi-two-dimensionalbreathing kagome lattice compound Pb(OF)Cu3(SeO3)2(NO3) using neutron diffraction and thermodynamicmeasurements. A long-range magnetic order emerges below the Neel temperature,TN=18 K, characterized bya propagating vectork=(0,0,1.5). Refinement analysis reveals that the copper moments display a noncoplanararrangement, with theccomponents parallelly aligned within the breathing kagome plane and antiparallellyaligned between the layers. In-plane moment components form a chiral "tail-chase" structure. The magneticorder is quickly suppressed under moderate external fields applied both within and perpendicular to the kagomeplane. Potential magnetic interactions that may be associated with the noncoplanar chiral magnetic structure arediscussed

引用

页数：9

共 50 条

[1] Pb(OF)Cu3(SeO3)2(NO3): a selenite fluoride nitrate with a breathing kagome lattice
Zhang, Mengsi
Zhao, Zhiying
Zhang, Wanwan
Li, Jinyang
Huang, Xiaoying
He, Zhangzhen
CHEMICAL COMMUNICATIONS, 2020, 56 (80) : 11965 - 11968
[2] PBCU3(OH)(NO3)(SEO3)3.1/2H2O AND PB2CU3O2(NO3)2(SEO3)2 - SYNTHESIS AND CRYSTAL-STRUCTURE
EFFENBERGER, H
MONATSHEFTE FUR CHEMIE, 1986, 117 (10): : 1099 - 1106
[3] Antiferroelectric instability in the kagome francisites Cu3 Bi(SeO3)2 O2X (X = Cl, Br)
Prishchenko, Danil A.
Tsirlin, Alexander A.
Tsurkan, Vladimir
Loidl, Alois
Jesche, Anton
Mazurenko, Vladimir G.
PHYSICAL REVIEW B, 2017, 95 (06)
[4] SYNTHESIS AND CRYSTAL-STRUCTURE OF PB2(NO2)(NO3)(SEO3)
EFFENBERGER, H
MONATSHEFTE FUR CHEMIE, 1987, 118 (02): : 211 - 216
[5] LATTICE-CONSTANTS OF CSH3(SEO3)2 AND CSD3(SEO3)2
ICHIKAWA, M
JOURNAL OF THE PHYSICAL SOCIETY OF JAPAN, 1986, 55 (04) : 1374 - 1379
[6] Co3(SeO3)(SO4)(OH)2: A Selenite-Sulfate Compound with a Distorted Kagome Lattice
Zhang, Mengsi
Song, Yujie
Zhao, Zhiying
Li, Jinyang
Zhang, Wanwan
Xie, Yaxin
Huang, Xing
Huang, Xiaoying
He, Zhangzhen
INORGANIC CHEMISTRY, 2020, 59 (12) : 8054 - 8060
[7] Syntheses and crystal structures of Pb(SeO3)2 and two modifications of Sn(SeO3)2
Steinhauser, Georg
Luef, Christoph
Wildner, Manfred
Giester, Gerald
JOURNAL OF ALLOYS AND COMPOUNDS, 2006, 419 (1-2) : 45 - 49
[8] Syntheses and crystal structures of Pb(SeO3)2 and two modifications of Sn(SeO3)2
Steinhauser, Georg
Luef, Christoph
Wildner, Manfred
Giester, Gerald
Journal of Alloys and Compounds, 2006, 419 (1-2): : 45 - 49
[9] Cu3(SeO3)2Cl2:: a new oxochloride of copper(II) and selenium(IV)
Millet, P
Bastide, B
Johnsson, M
SOLID STATE COMMUNICATIONS, 2000, 113 (12) : 719 - 723
[10] Syntheses, structures, and characterizations of a new second-order nonlinear optical material: Pb2(SeO3)(NO3)2
Meng, Chang-Yu
Geng, Lei
Chen, Wen-Ting
Wei, Ming-Fang
Dai, Kai
Lu, Hong-Yan
Cheng, Wen-Dan
JOURNAL OF ALLOYS AND COMPOUNDS, 2015, 640 : 39 - 44

← 1 2 3 4 5 →