Improved convolutional neural network-assisted laser-induced breakdown spectroscopy for identification of soil contamination types

被引:7
作者
Gou, Yujiang [1 ]
Fu, Xinglan [1 ]
Zhao, Shilin [1 ]
He, Panyu [1 ]
Zhao, Chunjiang [1 ,2 ]
Li, Guanglin [1 ]
机构
[1] Southwest Univ, Coll Engn & Technol, Chongqing 400716, Peoples R China
[2] Beijing Acad Agr & Forestry Sci, Natl Engn Res Ctr Informat Technol Agr, Beijing 100097, Peoples R China
关键词
Soil contamination types; Laser -induced breakdown spectroscopy; Convolutional neural network; Identification; RAPID CLASSIFICATION; HEAVY-METALS; SAMPLES; IMPACT; FOOD; SVM;
D O I
10.1016/j.sab.2024.106910
中图分类号
O433 [光谱学];
学科分类号
0703 ; 070302 ;
摘要
Identification of soil contamination types is of great scientific significance for soil remediation and environmental pollution control. However, traditional identification methods for soil determination are time-consuming, laborious, and complicated. Here, we proposed an accurate method for identifying soil contamination types based on laser-induced breakdown spectroscopy (LIBS) and an improved convolutional neural network (CNN) model. The spectral feature extraction-based multiple attention residual network (SFEMARNet) model was constructed to extract detailed features by spectral feature extraction (SFE) modules, and highlight useful features by multiple attention residual (MAR) modules in LIBS spectral data. In addition, deep learning models and machine learning models were used to identify the data. The results showed that the SFEMARNet model achieved an accuracy of 98.75% on the test set. The recall, precision, and F1-score of the models reached 98.78%, 98.75%, and 98.76%, respectively, which were significantly better than the three deep learning models and of four machine learning models. It seems that the SFEMARNet model combined with LIBS technology may be a potential method for the accurate identification of soil contamination types.
引用
收藏
页数:10
相关论文
共 46 条
[1]   Managing nutrients to mitigate soil pollution [J].
Bruulsema, Tom .
ENVIRONMENTAL POLLUTION, 2018, 243 :1602-1605
[2]   Elemental imaging using laser-induced breakdown spectroscopy: A new and promising approach for biological and medical applications [J].
Busser, Benoit ;
Moncayo, Samuel ;
Coll, Jean-Luc ;
Sancey, Lucie ;
Motto-Ros, Vincent .
COORDINATION CHEMISTRY REVIEWS, 2018, 358 :70-79
[3]   Deep spectral CNN for laser induced breakdown spectroscopy [J].
Castorena, Juan ;
Oyen, Diane ;
Ollila, Ann ;
Legget, Carey ;
Lanza, Nina .
SPECTROCHIMICA ACTA PART B-ATOMIC SPECTROSCOPY, 2021, 178
[4]   A novel bottom-viewed inductively coupled plasma-atomic emission spectrometry [J].
Chan, GCY ;
Chan, WT .
SPECTROCHIMICA ACTA PART B-ATOMIC SPECTROSCOPY, 2004, 59 (01) :41-58
[5]   Convolutional neural network as a novel classification approach for laser-induced breakdown spectroscopy applications in lithological recognition [J].
Chen, Junxi ;
Pisonero, Jorge ;
Chen, Sha ;
Wang, Xu ;
Fan, Qingwen ;
Duan, Yixiang .
SPECTROCHIMICA ACTA PART B-ATOMIC SPECTROSCOPY, 2020, 166
[6]   Deep learning with laser-induced breakdown spectroscopy (LIBS) for the classification of rocks based on elemental imaging [J].
Chen, Tong ;
Sun, Lanxiang ;
Yu, Haibin ;
Wang, Wei ;
Qi, Lifeng ;
Zhang, Peng ;
Zeng, Peng .
APPLIED GEOCHEMISTRY, 2022, 136
[7]   A solid phase extraction procedure for the determination of Cd(II) and Pb(II) ions in food and water samples by flame atomic absorption spectrometry [J].
Dasbasi, Teslima ;
Sacmaci, Serife ;
Ulgen, Ahmet ;
Kartal, Senol .
FOOD CHEMISTRY, 2015, 174 :591-596
[8]   Real-time classification of aluminum metal scrap with laser-induced breakdown spectroscopy using deep and other machine learning approaches [J].
Diaz-Romero, Dillam Jossue ;
Van den Eynde, Simon ;
Sterkens, Wouter ;
Eckert, Alexander ;
Zaplana, Isiah ;
Goedeme, Toon ;
Peeters, Jef .
SPECTROCHIMICA ACTA PART B-ATOMIC SPECTROSCOPY, 2022, 196
[9]   Discriminating crude oil grades using laser-induced breakdown spectroscopy [J].
El-Hussein, A. ;
Marzouk, A. ;
Harith, M. A. .
SPECTROCHIMICA ACTA PART B-ATOMIC SPECTROSCOPY, 2015, 113 :93-99
[10]   Rapid detection of chromium in different valence states in soil using resin selective enrichment coupled with laser-induced breakdown spectroscopy: From laboratory test to portable instruments [J].
Fu, Xinglan ;
Ma, Shixiang ;
Li, GuangLin ;
Guo, Lianbo ;
Dong, Daming .
SPECTROCHIMICA ACTA PART B-ATOMIC SPECTROSCOPY, 2020, 167