The ferroelectric and piezoelectric properties of (Hf1-xCex)O2 films on indium tin oxide/Pt/TiOx/SiO2/(100)Si substrates obtained using a no-heating radio-frequency magnetron sputtering deposition method

被引:1
作者
Chaya, Nachi [1 ]
Okamoto, Kazuki [1 ]
Hirai, Koji [1 ]
Yasuoka, Shinnosuke [1 ]
Inoue, Yukari [2 ]
Yamaoka, Wakiko [2 ]
Funakubo, Hiroshi [1 ]
机构
[1] Tokyo Inst Technol, Dept Mat Sci & Engn, Yokohama, Kanagawa 2268502, Japan
[2] TDK Corp, Tech Ctr, Ichikawa, Chiba 2728558, Japan
基金
日本学术振兴会;
关键词
no-heating processes; ferroelectric HfO2-based films; thick films; RF magnetron sputtering method; THIN-FILMS; CRYSTAL-STRUCTURE;
D O I
10.35848/1347-4065/ad3a71
中图分类号
O59 [应用物理学];
学科分类号
摘要
The effect of composition and film thickness on the ferroelectric and piezoelectric properties of (Hf1-xCex)O-2 films deposited without substrate heating was investigated. (Hf1-xCex)O-2 films with various x values (x = 0.07-0.27) and thickness (150-880 nm) were deposited via RF magnetron sputtering on indium tin oxide (ITO)/Pt/TiOx/SiO2/(100)Si substrates. The crystalline phases of the films were observed by X-ray diffraction. The measurements of electrical properties revealed ferroelectric phases in the x range of 0.11-0.21. The film with x = 0.16 exhibited the maximum remanent polarization (Pr) of 15 mu C cm(-2), as well as the highest effective piezoelectric coefficient. In addition, the ferroelectric and structural properties remained almost unchanged with increasing film thickness. Therefore, the no-heating deposition of ferroelectric (Hf1-xCex)O-2 films and their phase stability with respect to thickness were demonstrated in this study. This work provides a pathway for the deposition of ferroelectric (Hf1-xCex)O-2 films on flexible, wearable sensors. (c) 2024 The Japan Society of Applied Physics
引用
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页数:7
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