Compact realization of all-attosecond pump-probe spectroscopy

被引：18

作者：

Kretschmar, Martin ^{[1
]}

Svirplys, Evaldas ^{[1
]}

Volkov, Mikhail ^{[1
]}

Witting, Tobias ^{[1
]}

Nagy, Tamas ^{[1
]}

Vrakking, Marc J. J. ^{[1
]}

Schuette, Bernd ^{[1
]}

机构：

[1] Max Born Inst, Max Born Str 2A, D-12489 Berlin, Germany

来源：

SCIENCE ADVANCES | 2024年 / 10卷 / 08期

关键词：

REAL-TIME OBSERVATION; PULSES; DYNAMICS;

D O I：

10.1126/sciadv.adk9605

中图分类号：

O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];

学科分类号：

07 ; 0710 ; 09 ;

摘要：

The ability to perform attosecond-pump attosecond-probe spectroscopy (APAPS) is a longstanding goal in ultrafast science. While first pioneering experiments demonstrated the feasibility of APAPS, the low repetition rates (10 to 120 Hz) and the large footprints of existing setups have so far hindered the widespread exploitation of APAPS. Here, we demonstrate two-color APAPS using a commercial laser system at 1 kHz, straightforward post-compression in a hollow-core fiber, and a compact high-harmonic generation (HHG) setup. The latter enables the generation of intense extreme-ultraviolet (XUV) pulses by using an out-of-focus HHG geometry and by exploiting a transient blueshift of the driving laser in the HHG medium. Near-isolated attosecond pulses are generated, as demonstrated by one-color and two-color XUV-pump XUV-probe experiments. Our concept allows selective pumping and probing on extremely short timescales in many laboratories and permits investigations of fundamental processes that are not accessible by other pump-probe techniques.

引用

页数：7

共 54 条

[1] Tabletop nonlinear optics in the 100-eV spectral region [J].

Bergues, B. ;

Rivas, D. E. ;

Weidman, M. ;

Muschet, A. A. ;

Helml, W. ;

Guggenmos, A. ;

Pervak, V. ;

Kleineberg, U. ;

Marcus, G. ;

Kienberger, R. ;

Charalambidis, D. ;

Tzallas, P. ;

Schroeder, H. ;

Krausz, F. ;

Veisz, L. .

OPTICA, 2018, 5 (03) :237-242

[2]

Bloembergen N., 1973, Optics Communications, V8, P285, DOI 10.1016/0030-4018(73)90196-X

[3] Ultrafast electron dynamics in phenylalanine initiated by attosecond pulses [J].

Calegari, F. ;

Ayuso, D. ;

Trabattoni, A. ;

Belshaw, L. ;

De Camillis, S. ;

Anumula, S. ;

Frassetto, F. ;

Poletto, L. ;

Palacios, A. ;

Decleva, P. ;

Greenwood, J. B. ;

Martin, F. ;

Nisoli, M. .

SCIENCE, 2014, 346 (6207) :336-339

[4] Giant intermolecular decay and fragmentation of clusters [J].

Cederbaum, LS ;

Zobeley, J ;

Tarantelli, F .

PHYSICAL REVIEW LETTERS, 1997, 79 (24) :4778-4781

[5] ABSOLUTE OPTICAL OSCILLATOR-STRENGTHS FOR THE ELECTRONIC EXCITATION OF ATOMS AT HIGH-RESOLUTION .3. THE PHOTOABSORPTION OF ARGON, KRYPTON, AND XENON [J].

CHAN, WF ;

COOPER, G ;

GUO, X ;

BURTON, GR ;

BRION, CE .

PHYSICAL REVIEW A, 1992, 46 (01) :149-171

[6] Attosecond physics at the nanoscale [J].

Ciappina, M. F. ;

Perez-Hernandez, J. A. ;

Landsman, A. S. ;

Okell, W. A. ;

Zherebtsov, S. ;

Foerg, B. ;

Schoetz, J. ;

Seiffert, L. ;

Fennel, T. ;

Shaaran, T. ;

Zimmermann, T. ;

Chacon, A. ;

Guichard, R. ;

Zaier, A. ;

Tisch, J. W. G. ;

Marangos, J. P. ;

Witting, T. ;

Braun, A. ;

Maier, S. A. ;

Roso, L. ;

Krueger, M. ;

Hommelhoff, P. ;

Kling, M. F. ;

Krausz, F. ;

Lewenstein, M. .

REPORTS ON PROGRESS IN PHYSICS, 2017, 80 (05)

[7] Valence-shell photoionization of chlorinelike Ar+ ions [J].

Covington, A. M. ;

Aguilar, A. ;

Covington, I. R. ;

Hinojosa, G. ;

Shirley, C. A. ;

Phaneuf, R. A. ;

Alvarez, I. ;

Cisneros, C. ;

Dominguez-Lopez, I. ;

Sant'Anna, M. M. ;

Schlachter, A. S. ;

Ballance, C. P. ;

McLaughlin, B. M. .

PHYSICAL REVIEW A, 2011, 84 (01)

[8] Cold Target Recoil Ion Momentum Spectroscopy:: a 'momentum microscope' to view atomic collision dynamics [J].

Dörner, R ;

Mergel, V ;

Jagutzki, O ;

Spielberger, L ;

Ullrich, J ;

Moshammer, R ;

Schmidt-Böcking, H .

PHYSICS REPORTS-REVIEW SECTION OF PHYSICS LETTERS, 2000, 330 (2-3) :95-192

[9] Extreme-ultraviolet refractive optics [J].

Drescher, L. ;

Kornilov, O. ;

Witting, T. ;

Reitsma, G. ;

Monserud, N. ;

Rouzee, A. ;

Mikosch, J. ;

Vrakking, M. J. J. ;

Schuette, B. .

NATURE, 2018, 564 (7734) :91-+

[10] Time-resolved atomic inner-shell spectroscopy [J].

Drescher, M ;

Hentschel, M ;

Kienberger, R ;

Uiberacker, M ;

Yakovlev, V ;

Scrinzi, A ;

Westerwalbesloh, T ;

Kleineberg, U ;

Heinzmann, U ;

Krausz, F .

NATURE, 2002, 419 (6909) :803-807

← 1 2 3 4 5 6 →