Decoration of Bi2MoO6 nanosheets with NH2-UiO-66 for boosting visible-light photocatalytic activities

被引:1
作者
Hu, Qingsong [1 ]
Zhou, Ting [1 ]
Wang, Zhixin [1 ]
Liu, Yanbing [1 ]
Ye, Meng [1 ]
Zhang, Haijie [1 ]
Zhu, Xingwang [1 ]
Yi, Jianjian [1 ]
Xu, Yiqun [1 ]
机构
[1] Yangzhou Univ, Coll Environm Sci & Engn, 196 West Huayang Rd, Yangzhou 225127, Peoples R China
基金
中国博士后科学基金;
关键词
Bi2MoO6; nanosheets; Heterojunction interface; Charge carrier migration; Interface modulation; Visible-light irradiation; METAL-ORGANIC FRAMEWORK; DEGRADATION; REDUCTION; TETRACYCLINE; COMPOSITE; WATER;
D O I
10.1016/j.ica.2024.121979
中图分类号
O61 [无机化学];
学科分类号
070301 ; 081704 ;
摘要
Constructing heterostructured photocatalysts for organic contaminants elimination is promising in the area of environmental purification. For boosting the photocatalytic performance, modulating the heterojunction interface can enhance solar light utilization and facilitate the transporation of photoinduced charge carriers. In this research, octahedral NH2-UiO-66 nanoparticles with large surface area and wide light absorption range were prepared and further employed to in -situ construction of NH2-UiO-66/Bi2MoO6 nanocomposite. The optimized NH2-UiO-66/Bi2MoO6 nanocomposite displays enhanced photocatalytic activities in the elimination of rhodamine B (RhB) and tetracycline (TC). The corresponding degradation rate constant is about 4 and 1.76 times larger than that of individual Bi2MoO6. Combined with the photochemical and electrochemical results, it can be speculated that the higher photocatalytic performance is assigned to the accelerative photoinduced carrier transfer by the formation of well -contacted heterostructured interface. This study provides a theoretical basis for further developing organic-inorganic hybrid catalyst with significant improvement of photocatalytic properties in wastewater treatment.
引用
收藏
页数:8
相关论文
共 57 条
[1]   Surface defective g-C3N4-xClx with unique spongy structure by polarization effect for enhanced photocatalytic removal of organic pollutants [J].
Bai, Xiaojuan ;
Wang, Xuyu ;
Lu, Xiongwei ;
Liang, Yunjie ;
Li, Junqi ;
Wu, Liyuan ;
Li, Haiyan ;
Hao, Qiang ;
Ni, Bing-Jie ;
Wang, Chongchen .
JOURNAL OF HAZARDOUS MATERIALS, 2020, 398
[2]   Zr-based metal-organic frameworks: design, synthesis, structure, and applications [J].
Bai, Yan ;
Dou, Yibo ;
Xie, Lin-Hua ;
Rutledge, William ;
Li, Jian-Rong ;
Zhou, Hong-Cai .
CHEMICAL SOCIETY REVIEWS, 2016, 45 (08) :2327-2367
[3]   Floatable S-scheme Bi2WO6/C3N4/carbon fiber cloth composite for efficient water decontamination [J].
Cai, Mingjie ;
Liu, Yanping ;
Dong, Kexin ;
Chen, Xiaobo ;
Li, Shijie .
CHINESE JOURNAL OF CATALYSIS, 2023, 52 :239-251
[4]   Precise Design of Molecular Ferroelectrics with High T C and Tunable Band Gap by Molecular Modification [J].
Chen, Hao-Ran ;
Wan, Min ;
Li, Zi-Mu ;
Zhong, Wen-He ;
Ye, Si-Yu ;
Jia, Qiang-Qiang ;
Li, Jun-Yi ;
Chen, Li-Zhuang .
INORGANIC CHEMISTRY, 2023, 62 (30) :12018-12026
[5]   N-CND modified NH2-UiO-66 for photocatalytic CO2 conversion under visible light by a photo-induced electron transfer process [J].
Chen, Liyong ;
Yu, Fengyang ;
Shen, Xiaoshuang ;
Duan, Chunying .
CHEMICAL COMMUNICATIONS, 2019, 55 (33) :4845-4848
[6]   CO2 capture and photocatalytic reduction using bifunctional TiO2/MOF nanocomposites under UV-vis irradiation [J].
Crake, Angus ;
Christoforidis, Konstantinos C. ;
Kafizas, Andreas ;
Zafeiratos, Spyridon ;
Petit, Camille .
APPLIED CATALYSIS B-ENVIRONMENTAL, 2017, 210 :131-140
[7]   Sono-Magneto-Photocatalytic activity of Nd-BiFeO3/NiFe2O4 heterostructures [J].
Dhanalakshmi, Radhalayam ;
Sreekanth, T. V. M. ;
Denardin, Juliano ;
Rosaiah, P. ;
Sangaraju, Sambasivam ;
Yoo, Kisoo ;
Kim, Jonghoon .
MATERIALS LETTERS, 2023, 352
[8]   Atomically-thin Bi2MoO6 nanosheets with vacancy pairs for improved photocatalytic CO2 reduction [J].
Di, Jun ;
Zhao, Xiaoxu ;
Lian, Cheng ;
Ji, Mengxia ;
Xia, Jiexiang ;
Xiong, Jun ;
Zhou, Wu ;
Cao, Xingzhong ;
She, Yuanbin ;
Liu, Honglai ;
Loh, Kian Ping ;
Pennycook, Stephen J. ;
Li, Huaming ;
Liu, Zheng .
NANO ENERGY, 2019, 61 :54-59
[9]   Bismuth oxyhalide layered materials for energy and environmental applications [J].
Di, Jun ;
Xia, Jiexiang ;
Li, Huaming ;
Guo, Shaojun ;
Dai, Sheng .
NANO ENERGY, 2017, 41 :172-192
[10]   Partially etched Bi2O2CO3 by metal chloride for enhanced reactive oxygen species generation: A tale of two strategies [J].
Ding, Penghui ;
Di, Jun ;
Chen, Xiaoliu ;
Zhao, Junze ;
Gu, Kaizhi ;
Zhang, Yi ;
Yin, Sheng ;
Liu, Gaopeng ;
Xia, Jiexiang ;
Li, Huaming .
APPLIED CATALYSIS B-ENVIRONMENTAL, 2019, 245 :325-333