Nitrogen-doped graphene nanosheets as high efficient catalysts for oxygen reduction reaction

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CI SuQin WU YongMin ZOU JianPing TANG LongHua LUO ShengLian LI JingHong WEN ZhenHai Key Laboratory of Jiangxi Province for Ecological DiagnosisRemediation and Pollution ControlNanchang Hangkong UniversityNanchang China Department of ChemistryBeijing Key Laboratory for Microanalytical Methods and InstrumentationTsinghua UniversityBeijing China [1 ,2 ,1 ,2 ,1 ,2 ,1 ,1 ,330063 ,2 ,100084 ]
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It is of great significance in exploring alternative catalysts to platinum (Pt)-based materials for oxygen reduction reaction (ORR),because this reaction is invariably involved in various fuel cells and metal-air batteries.We herein reported the nitrogen doped graphene nanosheets (NGNSs) with pore volume of as high as 3.42 m 3 /g and investigated their potential application as ORR catalysts,it was demonstrated the NGNSs featured high activity,improved kinetics and excellent long-term stability for ORR.The NGNSs were successfully used as cathode catalysts of microbial fuel cells (MFCs) and performed even better than the commercial Pt/C (Pt 10%) catalysts at the maximum power output.
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页码:3065 / 3070
页数:6
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