SCANNING-TUNNELING-MICROSCOPY OBSERVATION AND THEORETICAL CALCULATION OF THE ADSORPTION OF ADENINE ON SI(100)2X1 SURFACES

被引：21

作者：

KASAYA, M ^{[1
]}

TABATA, H ^{[1
]}

KAWAI, T ^{[1
]}

机构：

[1] OSAKA UNIV,INST SCI & IND RES,IBARAKI,OSAKA 567,JAPAN

来源：

SURFACE SCIENCE | 1995年 / 342卷 / 1-3期

关键词：

AROMATICS; SCANNING TUNNELING MICROSCOPY; SEMIEMPIRICAL MODELS AND MODEL CALCULATIONS; SILICON; SURFACE STRUCTURE; MORPHOLOGY; ROUGHNESS; AND TOPOGRAPHY;

D O I：

10.1016/0039-6028(96)80001-X

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Scanning tunneling microscopy (STM) images of adenine molecules on Si(100)2 X 1 surfaces have shown for the first time that the adenine is adsorbed on a Si dimer row. The double bright molecular images are located on the neighboring two Si dimer rows and have ellipsoidal shapes. An extended Huckel molecular orbital calculation of the adenine adsorbed on the Si cluster gives the form of the hybridized orbital in this system. This calculation explains the adsorption site and the surface local density of states corresponding to the observed STM images.

引用

页码：215 / 223

页数：9

共 50 条

[21] Study of Si(001)4 x 2-Ga structure by scanning tunneling microscopy and ab initio calculation
Hara, Shinsuke
Kobayashi, Hidekazu
Irokawa, Katsumi
Fujishiro, Hiroki I.
Watanabe, Kazuyuki
Miki, Hirofumi
Kawazu, Akira
SURFACE SCIENCE, 2007, 601 (12) : 2415 - 2419
[22] Scanning tunneling microscopy/scanning tunneling spectroscopy of initial nitridation process of Si(100)-2 x 1 surfaces
Matsushita, D
Ikeda, H
Sakai, A
Zaima, S
Yasuda, Y
THIN SOLID FILMS, 2000, 369 (1-2) : 293 - 296
[23] Adsorption of elemental S on Si(100)-2x1 surfaces
Papageorgopoulos, A
Kamaratos, M
SURFACE SCIENCE, 1996, 352 : 364 - 368
[24] Room temperature adsorption of aniline (C6H5NH2) on Si(100)(2x1) observed with scanning tunneling microscopy
Rummel, RM
Ziegler, C
SURFACE SCIENCE, 1998, 418 (01) : 303 - 313
[25] ADSORPTION OF TIN ON THE GE(111)-C(2X8) SURFACE STUDIED WITH SCANNING-TUNNELING-MICROSCOPY AND PHOTOELECTRON-SPECTROSCOPY
GOTHELID, M
GREHK, TM
HAMMAR, M
KARLSSON, UO
FLODSTROM, SA
SURFACE SCIENCE, 1995, 328 (1-2) : 80 - 94
[26] Real-time scanning tunneling microscopy observation of Si(100)-(2x1)→(2xn)→c(4x4) structural phase transitions
Lin, DS
Wu, PH
SURFACE SCIENCE, 1998, 397 (1-3) : L273 - L279
[27] Atomic resolution imaging on Si(100)2x1 and Si(100)2x1:H surfaces with noncontact atomic force microscopy
Yokoyama, K
Ochi, T
Yoshimoto, A
Sugawara, Y
Morita, S
JAPANESE JOURNAL OF APPLIED PHYSICS PART 2-LETTERS & EXPRESS LETTERS, 2000, 39 (2A): : L113 - L115
[28] Thermal reactions of phosphine with Si(100): a combined photoemission and scanning-tunneling-microscopy study
Lin, DS
Ku, TS
Sheu, TJ
SURFACE SCIENCE, 1999, 424 (01) : 7 - 18
[29] Selenium adsorption on Cs-covered Si(100) 2x1 surfaces
Sotiropoulos, AK
Kamaratos, A
SOLID STATE COMMUNICATIONS, 2004, 129 (10) : 637 - 641
[30] Site conversion path and the kinetics of Ti on Si(001)-2x1 observed by scanning tunneling microscopy
Ishiyama, K
Taga, Y
Ichimiya, A
SURFACE SCIENCE, 1996, 349 (03) : 267 - 274

← 1 2 3 4 5 →