STUDIES OF THE TOTAL SYNTHESIS OF FREDERICAMYCIN-A - PREPARATION OF KEY PARTIAL STRUCTURES AND DEVELOPMENT OF AN INTERMOLECULAR ALKYNE CHROMIUM CARBENE COMPLEX BENZANNULATION CYCLIZATION APPROACH TO THE ABCD(E) RING-SYSTEM

被引：58

作者：

BOGER, DL

JACOBSON, IC

机构：

[1] Department of Chemistry and Medicinal Chemistry, Purdue University, West Lafayette

来源：

JOURNAL OF ORGANIC CHEMISTRY | 1990年 / 55卷 / 06期

关键词：

D O I：

10.1021/jo00293a043

中图分类号：

O62 [有机化学];

学科分类号：

070303 ; 081704 ;

摘要：

A study illustrating factors effecting the cyclization mode and regioselectivity of the alkyne-chromium carbene complex benzannulation cyclization reaction is detailed in development of a synthetic approach to the fredericamycin A ABCD(E) ring system. © 1990, American Chemical Society. All rights reserved.

引用

页码：1919 / 1928

页数：10

共 71 条

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[2] A MERCURY-MEDIATED ACYL MIGRATION IN A PINACOL-TYPE REARRANGEMENT - MODEL STUDIES TOWARD THE SYNTHESIS OF FREDERICAMYCIN-A
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[3] CONCERTED 1,2-CARBONYL MIGRATIONS IN ORGANIC-SYNTHESIS - A PRACTICAL SYNTHESIS OF SPIRO CYCLIC 1,3-DIKETONES
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[5] STUDIES ON THE TOTAL SYNTHESIS OF FREDERICAMYCIN-A - DEVELOPMENT OF AN INTERMOLECULAR ALKYNE-CHROMIUM CARBENE COMPLEX CYCLIZATION APPROACH TO THE ABCDE RING-SYSTEM
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[6] SYNTHESIS OF SPIROCYCLIC DIKETONES RELATED TO FREDERICAMYCIN-A
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[7] 1,3-DIPOLAR CYCLOADDITION REACTIONS OF TRANSITION-METAL CARBENE COMPLEXES AND THE FORMAL [3 + 2 + 1] PYRIDINANNULATION OF THE CYCLOADDUCTS
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[8] EFFICIENT PALLADIUM-MEDIATED SYNTHESIS OF A SPIROCYCLIC MODEL FOR FREDERICAMYCIN-A
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[J]. TETRAHEDRON LETTERS, 1987, 28 (02) : 171 - 174
[9] INTRAMOLECULAR ARYLATIONS OF SOFT ENOLATES CATALYZED BY ZEROVALENT PALLADIUM
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[J]. JOURNAL OF ORGANIC CHEMISTRY, 1988, 53 (17) : 4149 - 4151
[10] SYNTHESIS OF HETEROCYCLIC-COMPOUNDS RELATED TO FREDERICAMYCIN-A - THE CYCLOPENT[G]ISOQUINOLINE SYSTEM
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