Nonlinear Optical Properties of Functionalized DNA-CTMA complexes

被引:0
作者
Rau, Ileana [1 ]
Czaplicki, Robert [2 ,6 ]
Derkowska, Beata [3 ]
Grote, James G. [4 ]
Kajzar, Francois [1 ,2 ]
Krupka, Oksana [5 ]
Sahraoui, Bouchta [2 ]
机构
[1] Univ Politehn Bucuresti, Fac Appl Chem & Mat Sci, Str Polizu nr 1, Bucharest, Romania
[2] Univ Angers, Inst Sci Technol Mol Angers, MOLTECH Anjou UMR CNRS 6200, Equipe Interact Moleculaire Optique Non Lineaire, F-49045 Angers, France
[3] N Copernicus Univ, Inst Phys, PL-87100 Torun, Poland
[4] Air Force Res Lab Mat & Mfg Directorate, Wright Patterson AFB, OH 45433 USA
[5] Kiev Natl Taras Shevchenko Univ, Macromol Chem Dept, UA-01033 Kiev, Ukraine
[6] Tampere Univ Technol, Dept Phys, Opt Lab, FI-01033 Tampere, Finland
来源
NONLINEAR OPTICS QUANTUM OPTICS-CONCEPTS IN MODERN OPTICS | 2011年 / 42卷 / 3-4期
关键词
DNA; DNA-CTMA; functionalized DNA-CTMA; cobalt phthalocyanine; DR1; PCBM; NLO properties; third harmonic generation; DFWM; nonlinear absorption;
D O I
暂无
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Nonlinear optical properties of functionalized deoxyribonucleic acid (DNA) are reviewed and discussed. The studies were performed on thin films of DNA-CTMA and DNA-CTMA complex doped with: a charge transfer molecules DR1, pi conjugated with 2D (cobalt phthalocyanine) and 3D delocalization (C-60 derivative PCBM). The NLO properties of these compounds were studied by optical third harmonic generation at 1064.2 nm fundamental wavelength and by degenerate four wave mixing techniques at 532 nm by nanosecond and picosecond pulsed lasers, respectively. Fast THG chi((3))(- 3(w;w,w,w) as well as the real and imaginary parts of Kerr chi((3))(-w;w-w,w) susceptibilities were determined. The studies show that DNA, similarly as synthetic polymers, can be used as matrix for highly active NLO chromophores. A peculiar behaviour is observed at low dopant level which is interpreted as due to the two photon resonance and its position dependence on the doping mechanism.
引用
收藏
页码:283 / 323
页数:41
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