ENERGY-DEPENDENCE OF RATE COEFFICIENTS IN NUCLEATION THEORY

被引：0

作者：

BARRETT, JC

CLEMENT, CF

FORD, IJ

机构：

[1] Theoretical Studies Department, AEA Industrial Technology, Harwell Laboratory, Oxfordshire OX11 ORA

来源：

JOURNAL OF AEROSOL SCIENCE | 1991年 / 22卷

关键词：

D O I：

10.1016/S0021-8502(05)80033-3

中图分类号：

TQ [化学工业];

学科分类号：

0817 ;

摘要：

A general expression for the decay rate of a cluster of energy E is derived using equilibrium statistical mechanics. This decay rate is independent of the vapour temperature external to the cluster. Numerical results are presented for a model in which cluster molecules interact via a square well potential. The use of a Gaussian approximation for the equilibrium cluster energy distribution leads to an inaccurate form for the decay rate.

引用

页码：S55 / S58

页数：4

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