In this paper we present the preliminary results from a new experimental technique to synchronize the pulses from a mode-locked Nd-YAG laser to the light pulses in the VUV storage ring at the National Synchrotron Light Source (NSLS). We describe a method to electronically change the delay time between the laser pulses and the synchrotron pulses. We also illustrate a method to overlap the synchrotron pulses with the laser pulses in space and time. Preliminary results will be presented for two experiments.