RAMAN NONLINEAR SUSCEPTIBILITIES OF POLAR-MOLECULES

被引：1
|
作者：
KIRCHEVA, PP
机构：
[1] Inst. of Solid State Phys., Sofia, 1784
来源：
JOURNAL OF MOLECULAR STRUCTURE | 1992年 / 266卷
关键词：
D O I：
10.1016/0022-2860(92)80102-N
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
It is shown by means of density matrix formalism that the total expression for the third-order nonlinear susceptibility chi(3) (omega(4) = omega(1) - omega(2) + omega(3)) contains additional terms proportional to the differences or to the squared differences of permanent dipole moments of couples of energy levels. These new terms are interesting for some cases of electronic Raman transitions of polyatomic polar molecules, where their contribution to total Raman susceptibility could be significant.
引用
收藏
页码：429 / 434
页数：6
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