OBSERVATION OF THE FORBIDDEN 2ND-HARMONIC GENERATION IN RESONANCE WITH 2P WANNIER EXCITON IN ZNSE THIN-FILMS

被引:25
作者
MINAMI, F [1 ]
INOUE, K [1 ]
KATO, Y [1 ]
YOSHIDA, K [1 ]
ERA, K [1 ]
机构
[1] NATL INST RES INORGAN MAT,TSUKUBA,IBARAKI 305,JAPAN
关键词
D O I
10.1103/PhysRevLett.67.3708
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We have observed for the first time a drastic enhancement of the normally forbidden second-harmonic-generation signal when twice the incident photon energy is resonant with the excitation energy of a 2P exciton in thin ZnSe crystals. Measurements were performed, using a titanium-sapphire laser, at 4.2 K in such a geometrical configuration, x(zz, x or y)z or x(yy, x or y)z, that transitions are forbidden by the usual selection rules. The results are shown to be well accounted for in the framework of a time-dependent perturbation formalism.
引用
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页码:3708 / 3711
页数:4
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