NONUNIVERSALITY AND BREAKDOWN OF SCALING IN 2-SPECIES AGGREGATION WITH ANNIHILATION

被引:86
作者
KRAPIVSKY, PL
机构
[1] Central Aerohydrodynamic Institute, 140160 Moscow region
来源
PHYSICA A | 1993年 / 198卷 / 1-2期
关键词
D O I
10.1016/0378-4371(93)90187-9
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We study the kinetics of a simple model of aggregation with two distinct monomeric species in which irreversible bonding occurs only between like species and annihilation occurs between unlike species. In the mean-field approximation we find an unexpected kinetic behaviour which depends crucially on the ratio of reaction rates. For a relatively simple model of constant reaction rates, we investigate the corresponding rate equations and derive exact expressions for the exponents describing the kinetics of the model. It is observed that the kinetic behaviours of distinct species are quite different and that corresponding scaling exponents are also generally nonuniversal. Analytical solutions of the rate equations show that a modified scaling description, with different sets of exponents for light and heavy species, exists in systems with sufficiently weak annihilation; in systems with strong annihilation, the scaling for the cluster-mass distribution of the light species completely breaks down. A model with constant reaction rates of fusion and sum-kernel reaction rates of annihilation is also studied.
引用
收藏
页码:135 / 149
页数:15
相关论文
共 19 条
  • [1] NOTE ON THE KINETICS OF SYSTEMS MANIFESTING SIMULTANEOUS POLYMERIZATION-DEPOLYMERIZATION PHENOMENA
    BLATZ, PJ
    TOBOLSKY, AV
    [J]. JOURNAL OF PHYSICAL CHEMISTRY, 1945, 49 (02) : 77 - 80
  • [2] KINETICS OF FRAGMENTATION
    CHENG, Z
    REDNER, S
    [J]. JOURNAL OF PHYSICS A-MATHEMATICAL AND GENERAL, 1990, 23 (07): : 1233 - 1258
  • [3] STEADY-STATE DIFFUSION-CONTROLLED A+B-]O REACTIONS IN 2-DIMENSIONS AND 3-DIMENSIONS - RATE LAWS AND PARTICLE DISTRIBUTIONS
    CLEMENT, E
    SANDER, LM
    KOPELMAN, R
    [J]. PHYSICAL REVIEW A, 1989, 39 (12) : 6466 - 6471
  • [4] SOURCE-TERM AND EXCLUDED-VOLUME EFFECTS ON THE DIFFUSION-CONTROLLED A+B-]O REACTION IN ONE DIMENSION - RATE LAWS AND PARTICLE DISTRIBUTIONS
    CLEMENT, E
    SANDER, LM
    KOPELMAN, R
    [J]. PHYSICAL REVIEW A, 1989, 39 (12): : 6455 - 6465
  • [5] DRAKE R. L., 1972, TOPICS CURRENT AEROS
  • [6] Ernst MH, 1986, FRACTALS PHYSICS, P289
  • [7] KINETICS OF DROPLET GROWTH-PROCESSES - SIMULATIONS, THEORY, AND EXPERIMENTS
    FAMILY, F
    MEAKIN, P
    [J]. PHYSICAL REVIEW A, 1989, 40 (07): : 3836 - 3854
  • [8] FAMILY F, 1986, PHYS REV LETT, V57, P1875
  • [9] Frielander S., 1977, SMOKE DUST HAZE FUND
  • [10] FLUCTUATION-DOMINATED KINETICS IN DIFFUSION-CONTROLLED REACTIONS
    KANG, K
    REDNER, S
    [J]. PHYSICAL REVIEW A, 1985, 32 (01): : 435 - 447