IS DEPOLARIZED LIGHT SCATTERED FROM SIMPLE LIQUIDS MAINLY DOUBLE-SCATTERED

被引:19
作者
KEYES, T [1 ]
LADANYI, BM [1 ]
MADDEN, PA [1 ]
机构
[1] UNIV CAMBRIDGE,CHEM LAB,CAMBRIDGE CB2 1EW,ENGLAND
关键词
D O I
10.1016/0009-2614(79)80226-2
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The multiple-scattering series for depolarized light scattering from simple liquids is investigated. It is found that the leading term in the series, due to double-double scattering, is probably not large compared to double-triple (DT) scattering contributions. Existing theories, which neglect DT scattering, have concluded that the experimental data cannot be explained using the dipole-induced dipole (DID) model for the pair polarizability. It is suggested that a theory which includes DT scattering will not lead to rejection of the DID model. © 1979.
引用
收藏
页码:479 / 484
页数:6
相关论文
共 42 条
[31]   THEORY OF STATIC KERR EFFECT IN DENSE FLUIDS [J].
LADANYI, BM ;
KEYES, T .
MOLECULAR PHYSICS, 1977, 34 (06) :1643-1659
[32]   NEW METHOD FOR CALCULATION OF LIGHT-SCATTERING INTENSITIES - APPLICATION TO DEPOLARIZED SCATTERING FROM SIMPLE FLUIDS [J].
LADANYI, BM ;
KEYES, T .
MOLECULAR PHYSICS, 1976, 31 (06) :1685-1701
[33]   ROLE OF LOCAL FIELDS AND INTERPARTICLE PAIR CORRELATIONS IN LIGHT-SCATTERING BY DENSE FLUIDS .1. DEPOLARIZED INTENSITIES DUE TO ORIENTATIONAL FLUCTUATIONS [J].
LADANYI, BM ;
KEYES, T .
MOLECULAR PHYSICS, 1977, 33 (04) :1063-1097
[34]   CALCULATIONS OF ATOMIC AND MOLECULAR POLARIZABILITIES .1. METHODOLOGY AND APPLICATION TO AR-AR ASSOCIATION [J].
LALLEMAND, P ;
DAVID, DJ ;
BIGOT, B .
MOLECULAR PHYSICS, 1974, 27 (04) :1029-1043
[35]   POLARIZABILITY AND SECOND DIELECTRIC VIRAL COEFFICIENT OF INTERACTING HE ATOMS [J].
LIM, TK ;
LINDER, B ;
KROMHOUT, RA .
JOURNAL OF CHEMICAL PHYSICS, 1970, 52 (07) :3831-+
[36]   DYNAMIC MULTIPOLE POLARIZABILITIES OF H-2 AND HE AND LONG-RANGE INTERACTION COEFFICIENTS FOR H2-H2, H2-HE AND HE-HE [J].
MEYER, W .
CHEMICAL PHYSICS, 1976, 17 (01) :27-33
[37]   POLARIZABILITY OF INTERACTING ATOMS - RELATION TO COLLISION-INDUCED LIGHT-SCATTERING AND DIELECTRIC MODELS [J].
OBRIEN, EF ;
GUTSCHIC.VP ;
MCKOY, V ;
MCTAGUE, JP .
PHYSICAL REVIEW A, 1973, 8 (02) :690-696
[38]   GHOST ORBITALS AND BASIS SET EXTENSION EFFECTS [J].
OSTLUND, NS ;
MERRIFIELD, DL .
CHEMICAL PHYSICS LETTERS, 1976, 39 (03) :612-614
[39]   COLLISIONAL POLARIZABILITIES OF INERT-GASES 2ND-ORDER OVERLAP, EXCHANGE, AND CORRELATION EFFECTS [J].
OXTOBY, DW ;
GELBART, WM .
MOLECULAR PHYSICS, 1975, 30 (02) :535-547
[40]  
SHELTON DP, UNPUBLISHED