PERFORMANCE AND DURABILITY OF PT-MFI ZEOLITE CATALYST FOR SELECTIVE REDUCTION OF NITROGEN MONOXIDE IN ACTUAL DIESEL-ENGINE EXHAUST

被引:76
作者
IWAMOTO, M [1 ]
YAHIRO, H [1 ]
SHIN, HK [1 ]
WATANABE, M [1 ]
GUO, JW [1 ]
KONNO, M [1 ]
CHIKAHISA, T [1 ]
MURAYAMA, T [1 ]
机构
[1] ISHIKAWAJIMA HARIMA HEAVY IND CO LTD,KOTO KU,TOKYO 135,JAPAN
关键词
DIESEL ENGINE EXHAUST; MFI ZEOLITE; NITROGEN MONOXIDE; PLATINUM; SELECTIVE REDUCTION; ZEOLITES;
D O I
10.1016/0926-3373(94)00047-6
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Selective catalytic reduction of nitrogen monoxide (NO) by hydrocarbon in an oxidizing atmosphere has been studied over platinum-MFI zeolite (Pt-MFI) in synthesized or actual diesel engine exhaust gases. The activity of Pt-MFI in the synthesized gas, containing 10% water, changed in the early stage of the use, leveled off after 150-200 h, and remained constant for more than 800 h. The Pt-MFI catalyst also showed stable activity at 423-773 K and 10 000-150 000 h(-1) (gas hourly space velocity) in actual engine exhaust with light oil as a fuel. The degree of nitrogen monoxide reduction increased linearly upon addition of ethylene into the exhaust gas.
引用
收藏
页码:L1 / L6
页数:6
相关论文
共 9 条
[1]   HIGHLY SELECTIVE REDUCTION OF NITROGEN-OXIDES WITH HYDROCARBONS OVER H-FORM ZEOLITE CATALYSTS IN OXYGEN-RICH ATMOSPHERES [J].
HAMADA, H ;
KINTAICHI, Y ;
SASAKI, M ;
ITO, T ;
TABATA, M .
APPLIED CATALYSIS, 1990, 64 (1-2) :L1-L4
[2]  
HAMADA H, 1992, OCT P NAT M CAT SOC, P103
[3]   HIGH CATALYTIC ACTIVITY OF PLATINUM-ZSM-5 ZEOLITE BELOW 500-K IN WATER-VAPOR FOR REDUCTION OF NITROGEN MONOXIDE [J].
HIRABAYASHI, H ;
YAHIRO, H ;
MIZUNO, N ;
IWAMOTO, M .
CHEMISTRY LETTERS, 1992, (11) :2235-2236
[4]  
Iwamoto M., 1993, J AUTO ENG, V207, P23
[5]  
KONNO M, 1992, SAE T
[6]   PERFORMANCE OF PLATINUM-GROUP METAL-CATALYSTS FOR THE SELECTIVE REDUCTION OF NITROGEN-OXIDES BY HYDROCARBONS [J].
OBUCHI, A ;
OHI, A ;
NAKAMURA, M ;
OGATA, A ;
MIZUNO, K ;
OHUCHI, H .
APPLIED CATALYSIS B-ENVIRONMENTAL, 1993, 2 (01) :71-80
[7]  
SHIN HK, 1993, SHOKUBAI, V35, P402
[8]  
TRUEX TJ, 1992, PLATIN MET REV, V36, P2
[9]   SELECTIVE REDUCTION OF NITRIC-OXIDE OVER PLATINUM CATALYSTS IN THE PRESENCE OF SULFUR-DIOXIDE AND EXCESS OXYGEN [J].
ZHANG, G ;
YAMAGUCHI, T ;
KAWAKAMI, H ;
SUZUKI, T .
APPLIED CATALYSIS B-ENVIRONMENTAL, 1992, 1 (03) :L15-L20