PERFORMANCE AND DURABILITY OF PT-MFI ZEOLITE CATALYST FOR SELECTIVE REDUCTION OF NITROGEN MONOXIDE IN ACTUAL DIESEL-ENGINE EXHAUST

被引:76
作者
IWAMOTO, M [1 ]
YAHIRO, H [1 ]
SHIN, HK [1 ]
WATANABE, M [1 ]
GUO, JW [1 ]
KONNO, M [1 ]
CHIKAHISA, T [1 ]
MURAYAMA, T [1 ]
机构
[1] ISHIKAWAJIMA HARIMA HEAVY IND CO LTD,KOTO KU,TOKYO 135,JAPAN
关键词
DIESEL ENGINE EXHAUST; MFI ZEOLITE; NITROGEN MONOXIDE; PLATINUM; SELECTIVE REDUCTION; ZEOLITES;
D O I
10.1016/0926-3373(94)00047-6
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Selective catalytic reduction of nitrogen monoxide (NO) by hydrocarbon in an oxidizing atmosphere has been studied over platinum-MFI zeolite (Pt-MFI) in synthesized or actual diesel engine exhaust gases. The activity of Pt-MFI in the synthesized gas, containing 10% water, changed in the early stage of the use, leveled off after 150-200 h, and remained constant for more than 800 h. The Pt-MFI catalyst also showed stable activity at 423-773 K and 10 000-150 000 h(-1) (gas hourly space velocity) in actual engine exhaust with light oil as a fuel. The degree of nitrogen monoxide reduction increased linearly upon addition of ethylene into the exhaust gas.
引用
收藏
页码:L1 / L6
页数:6
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